Determination of the Conversion and Efficiency for CO2 in an Atmospheric Pressure Microwave Plasma Torch

被引：17

作者：

Wiegers, Katharina ^{[1
]}

Schulz, Andreas ^{[1
]}

Walker, Matthias ^{[1
]}

Tovar, Guenter E. M. ^{[1
]}

机构：

[1] Univ Stuttgart, Inst Interfacial Proc Engn & Plasma Technol IGVP, Pfaffenwaldring 31, D-70569 Stuttgart, Germany

来源：

CHEMIE INGENIEUR TECHNIK | 2022年 / 94卷 / 03期

关键词：

Atmospheric modular microwave plasma torch; CO2; conversion; Energy efficiency; Plasma technology; DISSOCIATION; OXYGEN;

D O I：

10.1002/cite.202100149

中图分类号：

TQ [化学工业];

学科分类号：

0817 ;

摘要：

In a 2.45 GHz plasma torch, carbon dioxide (CO2) has been converted into carbon monoxide (CO) and oxygen (O-2) at atmospheric pressure. The conversion and the efficiency of the plasma have been determined using two independent measuring methods: mass spectrometry and Fourier transform infrared absorption spectroscopy. The conversion depends on the measurement position in the exhaust gas duct. The conversion values at the beginning of the exhaust gas duct are significantly higher (maximum conversion is 22 %) than in the thermalized state at the end of the duct. In the cold, thermalized state of the gas, the maximum conversion rate is 8 % at 1.5 eV molecule(-1). The maximum efficiency of 25 % is achieved at approximatively 0.6 eV molecule(-1) operating at a microwave power of 0.48 kW and a mass flow of 12 slm CO2.

引用

页码：299 / 308

页数：10

共 41 条

[1]

[Anonymous], 2015, THE PARIS AGREEMENT

[2]

[Anonymous], 2009, QUADERA HTML HILFE

[3]

Asisov R. I., 1983, Proc. USSR Acad. Sci., V271, P94

[4] Carbon dioxide dissociation in a microwave plasma reactor operating in a wide pressure range and different gas inlet configurations [J].