Flexible and high-sensitivity sensor based on Ti3C2-MoS2 MXene composite for the detection of toxic gases

被引:91
作者
Van Thuan Le [1 ,2 ]
Vasseghian, Yasser [3 ]
Van Dat Doan [4 ]
Thi Thu Trang Nguyen [5 ]
Vo, Thu-Thao Thi [6 ]
Do, Ha Huu [7 ]
Khanh B Vu [8 ,11 ]
Vu, Quang Hieu [9 ]
Tran Dai Lam [5 ]
Tran, Vy Anh [10 ]
机构
[1] Duy Tan Univ, Ctr Adv Chem, Inst Res & Dev, 03 Quang Trung, Da Nang 55000, Vietnam
[2] Duy Tan Univ, Fac Nat Sci, 03 Quang Trung, Da Nang 55000, Vietnam
[3] Quchan Univ Technol, Dept Chem Engn, Quchan, Iran
[4] Ind Univ Ho Chi Minh City, Fac Chem Engn, Ho Chi Minh City 70000, Vietnam
[5] Vietnam Acad Sci & Technol, Inst Trop Technol, 18 Hoang Quoc Viet, Hanoi, Vietnam
[6] Gachon Univ, Coll BioNano Technol, Dept Food Sci & Biotechnol, Seongnam 13120, South Korea
[7] Chung Ang Univ, Sch Chem Engn & Mat Sci, 84 Heukseok Ro, Seoul 06974, South Korea
[8] Int Univ, Sch Biotechnol, Dept Chem Engn, Ho Chi Minh City, Vietnam
[9] Nguyen Tat Thanh Univ, NTT Hitech Inst, 300A Nguyen Tat Thanh,Ward 13,Dist 4, Ho Chi Minh City, Vietnam
[10] Gachon Univ, Dept Chem & Biol Engn, 1342 Seongnamdaero, Seongnam Si 13120, South Korea
[11] Vietnam Natl Univ, Ho Chi Minh City, Vietnam
关键词
Gas sensor; Ti3C2; MXene; Multigas-detection; MoS2; DRUG-RELEASE; MOS2;
D O I
10.1016/j.chemosphere.2021.133025
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
It is vital to have high sensitivity in gas sensors to allow the exact detection of dangerous gases in the air and at room temperature. In this study, we used 2D MXenes and MoS2 materials to create a Ti3C2-MoS2 composite with high metallic conductivity and a wholly functionalized surface for a significant signal. At room temperature, the Ti3C2-MoS2 composite demonstrated clear signals, cyclic response curves to NO2 gas, and gas concentrationdependent. The sensitivities of the standard Ti3C2-MoS2 (TM_2) composite (20 wt% MoS2) rose dramatically to 35.8%, 63.4%, and 72.5% when increasing NO2 concentrations to 10 ppm, 50 ppm, and 100 ppm, respectively. In addition, the composite showed reaction signals to additional hazardous gases, such as ammonia and methane. Our findings suggest that highly functionalized metallic sensing channels could be used to construct multigas-detecting sensors that are very sensitive in air and at room temperature.
引用
收藏
页数:8
相关论文
共 39 条
  • [1] Experimental and Theoretical Advances in MXene-Based Gas Sensors
    Aghaei, Sadegh Mehdi
    Aasi, Aref
    Panchapakesan, Balaji
    [J]. ACS OMEGA, 2021, 6 (04): : 2450 - 2461
  • [2] 2D Ti3C2 MXene/WO3 Hybrid Architectures for High-Rate Supercapacitors
    Ambade, Swapnil B.
    Ambade, Rohan B.
    Eom, Wonsik
    Noh, Sung Hyun
    Kim, Seung Hun
    Han, Tae Hee
    [J]. ADVANCED MATERIALS INTERFACES, 2018, 5 (24):
  • [3] Targeted and controlled drug delivery by multifunctional mesoporous silica nanoparticles with internal fluorescent conjugates and external polydopamine and graphene oxide layers
    Anh-Vy Tran
    Shim, KyuHwan
    Thu-Thao Vo Thi
    Kook, Jeong-Keun
    An, Seong Soo A.
    Lee, Sang-Wha
    [J]. ACTA BIOMATERIALIA, 2018, 74 : 397 - 413
  • [4] Vertically aligned MoS2 on Ti3C2 (MXene) as an improved HER catalyst
    Attanayake, Nuwan H.
    Abeyweera, Sasitha C.
    Thenuwara, Akila C.
    Anasori, Babak
    Gogotsi, Yury
    Sun, Yugang
    Strongin, Daniel R.
    [J]. JOURNAL OF MATERIALS CHEMISTRY A, 2018, 6 (35) : 16882 - 16889
  • [5] Charge-transfer-based Gas Sensing Using Atomic-layer MoS2
    Cho, Byungjin
    Hahm, Myung Gwan
    Choi, Minseok
    Yoon, Jongwon
    Kim, Ah Ra
    Lee, Young-Joo
    Park, Sung-Gyu
    Kwon, Jung-Dae
    Kim, Chang Su
    Song, Myungkwan
    Jeong, Yongsoo
    Nam, Kee-Seok
    Lee, Sangchul
    Yoo, Tae Jin
    Kang, Chang Goo
    Lee, Byoung Hun
    Ko, Heung Cho
    Ajayan, Pulickel M.
    Kim, Dong-Ho
    [J]. SCIENTIFIC REPORTS, 2015, 5 : 8052
  • [6] 2D layered MoS2 based gas sensor for indoor pollutant formaldehyde gas sensing applications
    Choi, Gyu Jin
    Mishra, Rajneesh Kumar
    Gwag, Jin Seog
    [J]. MATERIALS LETTERS, 2020, 264
  • [7] Ti3C2Tx MXene sensor for rapid Hg2+ analysis in high salinity environment
    Hao, Sibei
    Liu, Chengbin
    Chen, Xiaoyan
    Zong, Boyang
    Wei, Xiaojie
    Li, Qiuju
    Qin, Hehe
    Mao, Shun
    [J]. JOURNAL OF HAZARDOUS MATERIALS, 2021, 418
  • [8] Rational Design of MoS2/C3N4 Hybrid Aerogel with Abundant Exposed Edges for Highly Sensitive NO2 Detection at Room Temperature
    Ikram, Muhammad
    Lv, He
    Liu, Zhuo
    Khan, Mawaz
    Liu, Lujia
    Raziq, Fazal
    Bai, Xue
    Ullah, Mohib
    Zhang, Yang
    Shi, Keying
    [J]. CHEMISTRY OF MATERIALS, 2020, 32 (17) : 7215 - 7225
  • [9] Facile synthesis of Ag-ZnO core-shell nanostructures with enhanced photocatalytic activity
    Kadam, A. N.
    Bhopate, D. P.
    Kondalkar, V. V.
    Majhi, S. M.
    Bathula, C. D.
    Anh-Vy Tran
    Lee, Sang-Wha
    [J]. JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY, 2018, 61 : 78 - 86
  • [10] Metallic Ti3C2TX MXene Gas Sensors with Ultrahigh Signal-to-Noise Ratio
    Kim, Seon Joon
    Koh, Hyeong-Jun
    Ren, Chang E.
    Kwon, Ohmin
    Maleski, Kathleen
    Cho, Soo-Yeon
    Anasori, Babak
    Kim, Choong-Ki
    Choi, Yang-Kyu
    Kim, Jihan
    Gogotsi, Yury
    Jung, Hee-Tae
    [J]. ACS NANO, 2018, 12 (02) : 986 - 993