Tip-enhanced Raman spectroscopy: From concepts to practical applications

被引：60
作者：
Jiang, Nan [1 ]
Kurouski, Dmitry [2 ]
Pozzi, Eric A. [2 ]
Chiang, Naihao [3 ]
Hersam, Mark C. [2 ,3 ,4 ]
Van Duyne, Richard P. [2 ,3 ]
机构：
[1] Univ Illinois, Dept Chem, Chicago, IL 60607 USA
[2] Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA
[3] Northwestern Univ, Appl Phys Grad Program, Evanston, IL 60208 USA
[4] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA
来源：
CHEMICAL PHYSICS LETTERS | 2016年 / 659卷
基金：
美国国家科学基金会;
关键词：
SCANNING-TUNNELING-MICROSCOPY; FEMTOSECOND-STIMULATED RAMAN; SINGLE-MOLECULE; ATOMIC-RESOLUTION; IN-SITU; ELECTROCHEMICAL INTERFACES; CHEMICAL-ANALYSIS; CARBON NANOTUBES; SCATTERING; SURFACE;
D O I：
10.1016/j.cplett.2016.06.035
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Tip-enhanced Raman spectroscopy (TERS) is a powerful technique that integrates the vibrational fingerprinting of Raman spectroscopy and the sub-nanometer resolution of scanning probe microscopy (SPM). As a result, TERS is capable of obtaining chemical maps of analyzed specimens with exceptional lateral resolution. This is extremely valuable for the study of interactions between molecules and substrates, in addition to structural characterization of biological objects, such as viruses and amyloid fibrils, 2D polymeric materials, and monitoring electrochemical and photo-catalytic processes. In this mini review, we discuss the most significant advances of TERS, including: super high resolution chemical imaging, monitoring of catalytic processes, incorporation of pulsed-excitation techniques, single-site electrochemistry, biosensing, and art conservation. We begin with a short overview of TERS, comparing it with other surface analytical techniques, followed by an overview of recent developments and future applications in TERS. (C) 2016 Elsevier B.V. All rights reserved.
引用
收藏
页码：16 / 24
页数：9
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