Waste tea residue as a low cost adsorbent for removal of hydralazine hydrochloride pharmaceutical pollutant from aqueous media: An environmental remediation

被引:61
作者
Patil, Chandrashekhar S. [1 ,2 ,3 ]
Gunjal, Datta B. [2 ]
Naik, Vaibhav M. [2 ]
Harale, Namdev S. [1 ]
Jagadale, Suryabala D. [1 ]
Kadam, Abhijit N. [4 ]
Patil, Pramod S. [1 ]
Kolekar, Govind B. [2 ]
Gore, Anil H. [2 ,3 ]
机构
[1] Shivaji Univ, Sch Nanosci & Technol, Kolhapur 416004, MS, India
[2] Shivaji Univ, Dept Chem, Fluorescence Spect Res Lab, Kolhapur 416004, MS, India
[3] Rajarshi Chhatrapati Shahu Coll, Dept Chem, Kolhapur 416005, MS, India
[4] Gachon Univ, Dept Chem & Biol Engn, Nanoparticles Proc Lab, Seongnam City 461701, South Korea
关键词
Waste tea residue; Hydralazine hydrochloride; Adsorptive removal; Pharmaceutical pollutant; Water treatment; Environmental remediation; DRINKING-WATER TREATMENT; HEAVY-METAL IONS; ACTIVATED CARBON; POTENTIAL USE; ADSORPTION; DYE; BIOMASS; SULFAMETHOXAZOLE; TETRACYCLINE; DICLOFENAC;
D O I
10.1016/j.jclepro.2018.09.140
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Herein, we introduced simple, cheap, cost-effective and sustainable kitchen waste tea residue as an adsorbent. As per the literature survey, all the adsorbents have been used for wastewater treatment only as activated form. The first time, we have used similar material without any complicated activation process for the removal of pharmaceutical pollutant and it shows superior results than the existing materials which are the most attractive part of this work. It has shown an effective, low cost bio-sorbent to remove Hydralazine hydrochloride pharmaceutical pollutant from wastewater in aqueous media. The adsorbent waste tea residue was characterized by using Scanning Electron Microscopy, Brunauer-Emmett-Teller and Fourier transform infrared spectroscopy. The effect of pH, adsorbent dosage, contact time, and initial concentration on Hydralazine hydrochloride removal were also systematically studied. The adsorption process was studied using experimental data were fitted in both isotherms models. The maximum adsorption capacity of waste tea residue was found to be q(e) = 131.63 mg g(-1) which is higher than the reported value. Furthermore, developed adsorbent was practically used to remove pharmaceutical pollutants from real samples (hospital and river wastewater) spiked with Hydralazine hydrochloride. Therefore, the waste tea residue displays the great potential to improve the quality of water contaminated with different type's pharmaceuticals in the environment. (C) 2018 Elsevier Ltd. All rights reserved.
引用
收藏
页码:407 / 418
页数:12
相关论文
共 58 条
[1]   Adsorption of cephalexin onto activated carbons from Albizia lebbeck seed pods by microwave-induced KOH and K2CO3 activations [J].
Ahmed, Muthanna J. ;
Theydan, Samar K. .
CHEMICAL ENGINEERING JOURNAL, 2012, 211 :200-207
[2]   Pine sawdust biomass and biochars at different pyrolysis temperatures change soil redox processes [J].
Awad, Yasser Mahmoud ;
Ok, Yong Sik ;
Abrigata, Jens ;
Beiyuan, Jingzi ;
Beckers, Felix ;
Tsang, Daniel C. W. ;
Rinklebe, Joerg .
SCIENCE OF THE TOTAL ENVIRONMENT, 2018, 625 :147-154
[3]   The interaction of carboxylic acids with aluminium oxides: journeying from a basic understanding of alumina nanoparticles to water treatment for industrial and humanitarian applications [J].
Barron, Andrew R. .
DALTON TRANSACTIONS, 2014, 43 (22) :8127-8143
[4]   Life cycle analysis of hydrothermal carbonization of olive mill waste: Comparison with current management approaches [J].
Benavente, Veronica ;
Fullana, Andres ;
Berge, Nicole D. .
JOURNAL OF CLEANER PRODUCTION, 2017, 142 :2637-2648
[5]   Kinetics and thermodynamics of cadmium ion removal by adsorption onto nano zerovalent iron particles [J].
Boparai, Hardiljeet K. ;
Joseph, Meera ;
O'Carroll, Denis M. .
JOURNAL OF HAZARDOUS MATERIALS, 2011, 186 (01) :458-465
[6]   Potential use of alkaline treated algae waste biomass as sustainable biosorbent for clean recovery of cadmium(II) from aqueous media: batch and column studies [J].
Bulgariu, Dumitru ;
Bulgariu, Laura .
JOURNAL OF CLEANER PRODUCTION, 2016, 112 :4525-4533
[7]   Production of adsorbents by pyrolysis of paper mill sludge and application on the removal of citalopram from water [J].
Calisto, Vania ;
Ferreira, Catarina I. A. ;
Santos, Sergio M. ;
Victoria Gil, Maria ;
Otero, Marta ;
Esteves, Valdemar I. .
BIORESOURCE TECHNOLOGY, 2014, 166 :335-344
[8]   THE ADSORPTION OF HEAVY-METALS ONTO HYDROUS ACTIVATED CARBON [J].
CORAPCIOGLU, MO ;
HUANG, CP .
WATER RESEARCH, 1987, 21 (09) :1031-1044
[9]   Non-conventional low-cost adsorbents for dye removal: A review [J].
Crini, G .
BIORESOURCE TECHNOLOGY, 2006, 97 (09) :1061-1085
[10]   Artemisia vulgaris-derived mesoporous honeycomb-shaped activated carbon for ibuprofen adsorption [J].
Dubey, Shashi Prabha ;
Dwivedi, Amarendra Dhar ;
Sillanpaa, Mika ;
Gopal, Krishna .
CHEMICAL ENGINEERING JOURNAL, 2010, 165 (02) :537-544