Mitigation studies of carbon corrosion by optimizing the opening size of the cathode outlet in a proton exchange membrane fuel cell with dead-ended anode

被引:75
|
作者
Chen, Ben [1 ,2 ]
Wang, Jun [1 ]
Yang, Tianqi [2 ]
Cai, Yonghua [2 ]
Pan, Mu [1 ]
Tu, Zhengkai [1 ,3 ]
Zhang, Caizhi [3 ]
Chan, Siew Hwa [3 ]
Yu, Yi [4 ]
机构
[1] Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, Wuhan 430070, Peoples R China
[2] Wuhan Univ Technol, Hubei Key Lab Adv Technol Automot Components, Wuhan 430070, Peoples R China
[3] Nanyang Technol Univ, Energy Res Inst, 50 Nanyang Ave, Singapore 637553, Singapore
[4] SAIC Motor, Res & Adv Technol Dept, Shanghai 201804, Peoples R China
关键词
Proton exchange membrane fuel cell; Dead-ended; Mitigation; Carbon corrosion; FLOW-FIELD; WATER MANAGEMENT; GAS CHANNELS; PEMFC; PERFORMANCE; OPTIMIZATION; DEGRADATION; STARVATION; OPERATION; TRANSPORT;
D O I
10.1016/j.enconman.2016.04.043
中图分类号
O414.1 [热力学];
学科分类号
摘要
Water management is the key issue for the cathode in a proton exchange membrane fuel cell, nearly all the humidified and generated water is flow out of the fuel cell through the outlet of the cathode. Cathode flooding can lead to dramatic performance decay and irrecoverable material degradation in fuel cell. Therefore, optimization design at the cathode outlet is a significant technical challenge for the performance and lifetime enhancement for fuel cell. To address this problem, this study optimized the opening size at cathode outlet of the fuel cell that operates under dead-ended anode mode. The designed cells were continuously operated for 100 h under dead-ended anode mode and the effect of opening size in cathode outlet on cell performance has been investigated. It was found that, with the increase in opening size at cathode outlet, the flooding electrode and the consequent carbon corrosion in catalyst layer can be substantially suppressed. (C) 2016 Elsevier Ltd. All rights reserved.
引用
收藏
页码:60 / 66
页数:7
相关论文
共 50 条
  • [31] Optimization of the performance, operation conditions and purge rate for a dead-ended anode proton exchange membrane fuel cell using an analytical model
    Dashti, Isar
    Asghari, Saeed
    Goudarzi, Mohammad
    Meyer, Quentin
    Mehrabani-Zeinabad, Arjomand
    Brett, Dan J. L.
    ENERGY, 2019, 179 : 173 - 185
  • [32] Investigation of self-humidified and dead-ended anode proton exchange membrane fuel cell performance using electrochemical impedance spectroscopy
    Asgharr, Saeed
    Khorasani, Mohammad Reza Ashraf
    Dashti, Isar
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2016, 41 (28) : 12347 - 12357
  • [33] A comprehensive system-level model for performance evaluation of proton exchange membrane fuel cell system with dead-ended anode mode
    Hu, B. B.
    Qu, Z. G.
    Tao, W. Q.
    APPLIED ENERGY, 2023, 347
  • [34] Dynamic evolutions of local current density and water-gas distribution of proton exchange membrane fuel cell with dead-ended anode
    Yang, Guanghua
    Deng, Qihao
    Zhou, Yu
    Chen, Wenshang
    Chen, Ben
    ENERGY CONVERSION AND MANAGEMENT, 2023, 298
  • [35] Modeling and analysis of water droplet dynamics in the dead-ended anode gas channel for proton exchange membrane fuel cells
    Shao, Heng
    Qiu, Diankai
    Peng, Linfa
    Yi, Peiyun
    Lai, Xinmin
    RENEWABLE ENERGY, 2019, 138 : 842 - 851
  • [36] Detecting cathode corrosion in polymer electrolyte membrane fuel cells in dead-ended anode mode via alternating current impedance
    Ge, N.
    Chevalier, S.
    Muirhead, D.
    Banerjee, R.
    Lee, J.
    Liu, H.
    Shrestha, P.
    Fahy, K.
    Lee, C. H.
    Aoki, T.
    Tabuchi, Y.
    Bazylak, A.
    JOURNAL OF POWER SOURCES, 2019, 439
  • [37] A transient heat and mass transfer CFD simulation for proton exchange membrane fuel cells (PEMFC) with a dead-ended anode channel
    Peng, Yeping
    Mahyari, Hamed Moradi
    Moshfegh, Abouzar
    Javadzadegan, Ashkan
    Toghraie, Davood
    Shams, Mehrzad
    Rostami, Sara
    INTERNATIONAL COMMUNICATIONS IN HEAT AND MASS TRANSFER, 2020, 115
  • [38] Visualization study on enhancing water transport of proton exchange membrane fuel cells with a dead-ended anode by generating fluctuating flow at anode compartment
    Zhao, Jing
    Jian, Qifei
    Huang, Zipeng
    ENERGY CONVERSION AND MANAGEMENT, 2020, 206
  • [39] Nitrogen Front Evolution in Purged Polymer Electrolyte Membrane Fuel Cell with Dead-Ended Anode
    Siegel, Jason B.
    Bohac, Stanislav V.
    Stefanopoulou, Anna G.
    Yesilyurt, Serhat
    JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2010, 157 (07) : B1081 - B1093
  • [40] In situ analysis of voltage degradation in a polymer electrolyte membrane fuel cell with a dead-ended anode
    Chevalier, S.
    Ge, N.
    Lee, J.
    Antonacci, P.
    Yip, R.
    George, M. G.
    Liu, H.
    Banerjee, R.
    Fazeli, M.
    Bazylak, A.
    ELECTROCHEMISTRY COMMUNICATIONS, 2015, 59 : 16 - 19