Study of iodine releases from epoxy and polyurethane paints under irradiation and development of a new model of iodine-Epoxy paint interactions for PHEBUS and PWR severe accident applications

被引:12
作者
Bosland, Loic [1 ]
Colombani, Juliette [1 ]
机构
[1] PSN RES, Inst Radioprotect & Surete Nucl, Cadarache BP 3, F-13115 St Paul Les Durance, France
关键词
Iodine; Epoxy paint; Polyurethane paint; Kinetics; Severe accident; PHEBUS-FPT-3; PROJECT RADIOLYTIC OXIDATION; MOLECULAR-IODINE; INTEGRAL CODE; ASTEC; CONTAINMENT; BEHAVIOR; FP; RADIOCHEMISTRY; DESTRUCTION; FEATURES;
D O I
10.1007/s10967-017-5458-9
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
A new model of iodine-Epoxy paint interaction under irradiation has been developed with new relevant data to better reproduce and predict how much iodine could be released in the environment in case of a severe accident in a Pressurized Water Reactor. Its application to the modelling of volatile iodine behaviour in PHEBUS-FPT-3 test is presented and shows that other phenomena might govern the iodine volatility in the mid and long term. A broader analysis of the gaseous iodine behaviour is finally presented, highlighting the need to identify and model new gaseous chemical reactions that might play a significant role on iodine volatility.
引用
收藏
页码:1121 / 1140
页数:20
相关论文
共 54 条
[1]  
Aleksandrov A. B., 1995, Thermal Engineering, V42, P991
[2]  
[Anonymous], P AMSE JSME ICONE
[3]  
Barnes RH, 1968, BMI1829 UNCL
[4]  
BARTONICEK B, 1986, RADIAT PHYS CHEM, V28, P591
[5]  
Bartonicek B, 1987, P 4 WORK M RAD INT L, P491
[6]  
Belval-Haltier E, 1999, OECD WORKSH IOD ASP, P103
[7]   Phebus-FP:: Results and significance for plant safety in Switzerland [J].
Birchley, J ;
Haste, T ;
Bruchertseifer, H ;
Cripps, R ;
Güntay, S ;
Jäckel, B .
NUCLEAR ENGINEERING AND DESIGN, 2005, 235 (15) :1607-1633
[8]   Iodine-paint interactions during nuclear reactor severe accidents [J].
Bosland, L. ;
Dickinson, S. ;
Glowa, G. A. ;
Herranz, L. E. ;
Kim, H. C. ;
Powers, D. A. ;
Salay, M. ;
Tietze, S. .
ANNALS OF NUCLEAR ENERGY, 2014, 74 :184-199
[9]   MODELING AND INTERPRETATION OF IODINE BEHAVIOR IN PHEBUS FPT-1 CONTAINMENT WITH ASTEC AND COCOSYS CODES [J].
Bosland, L. ;
Weber, G. ;
Klein-Hessling, W. ;
Girault, N. ;
Clement, B. .
NUCLEAR TECHNOLOGY, 2012, 177 (01) :36-62
[10]   PARIS project: Radiolytic oxidation of molecular iodine in containment during a nuclear reactor severe accident: Part 2. Formation and destruction of iodine oxides compounds under irradiation - Experimental results modelling [J].
Bosland, L. ;
Funke, F. ;
Langrock, G. ;
Girault, N. .
NUCLEAR ENGINEERING AND DESIGN, 2011, 241 (09) :4026-4044