Personal exposure to UFP in different micro-environments and time of day

被引:23
作者
de Kluizenaar, Y. [1 ]
Kuijpers, E. [1 ]
Eekhout, I. [1 ]
Voogt, M. [1 ]
Vermeulen, R. C. H. [2 ]
Hoek, G. [2 ]
Sterkenburg, R. P. [1 ]
Pierik, F. H. [1 ]
Duyzer, J. H. [1 ]
Meijer, E. W. [1 ]
Pronk, A. [1 ]
机构
[1] Netherlands Org Appl Sci Res TNO, POB 96800, NL-2509 JE The Hague, Netherlands
[2] IRAS, POB 80178, NL-3508 TD Utrecht, Netherlands
关键词
Air pollution; Ultrafine particulate matter; Personal exposure monitoring; GPS; Micro environments; Time activity patterns; ULTRAFINE PARTICLES; PARTICULATE MATTER; AIR-POLLUTION; CHEMICAL-COMPOSITION; SIZE; INDOOR; PM2.5; COMPARABILITY; CHILDREN; PM10;
D O I
10.1016/j.buildenv.2017.06.022
中图分类号
TU [建筑科学];
学科分类号
0813 ;
摘要
Particulate matter exposure may cause adverse health effects. Although ultrafine particulate matter (UFP) is hypothesised to be particularly health relevant, the number of studies into personal UFP exposure is limited. Aim: To increase insight where and when most UFP exposure occurs, in terms of exposure levels and peaks in microenvironments, time of day and activities, to support development of abatement strategies to reduce exposure. Methods: UFP exposure and GPS tracks were recorded continuously for 5 days in 12 healthy volunteers. GPS data was processed to assign context information, and linked to UFP data. Results: Participants spent most time indoors (>90%), mainly at home (approx. 80%). Mean particle number concentration (particles/cm(3)) was highest in motorized transport (20.5 x 10(3)), followed by other indoor environments (16.5 x 10(3)), and lower at home (11.2 x 10(3)) and walking outdoors (9.0 x 10(3)). Due to the large proportion of time spent indoors, exposure indoors contributed most to total exposure (nearly 90%). Exposure during motorized transport showed a speed dependency, most likely linked to exposure on larger busier roads. Using a 95th percentile cut-off for concentration elevations lasting at least 5 min for peak-detection, 98 peaks were identified, mainly during daytime. These contributed substantially to total exposure (25%) while accounting for only 3.4% of total time. Of this peak contribution 88% occurred indoors (mainly at home) and 12% outdoors. Conclusions: UFP exposure shows clear differences between microenvironments. Peaks contribute substantially to total exposure. Measures to prevent peak exposures could contribute to substantial exposure reduction. (C) 2017 Elsevier Ltd. All rights reserved.
引用
收藏
页码:237 / 246
页数:10
相关论文
共 39 条
[1]   Emissions and indoor concentrations of particulate matter and its specific chemical components from cooking: A review [J].
Abdullahi, Karimatu L. ;
Delgado-Saborit, Juana Maria ;
Harrison, Roy M. .
ATMOSPHERIC ENVIRONMENT, 2013, 71 :260-294
[2]   Particulate Matter Air Pollution and Cardiovascular Disease An Update to the Scientific Statement From the American Heart Association [J].
Brook, Robert D. ;
Rajagopalan, Sanjay ;
Pope, C. Arden, III ;
Brook, Jeffrey R. ;
Bhatnagar, Aruni ;
Diez-Roux, Ana V. ;
Holguin, Fernando ;
Hong, Yuling ;
Luepker, Russell V. ;
Mittleman, Murray A. ;
Peters, Annette ;
Siscovick, David ;
Smith, Sidney C., Jr. ;
Whitsel, Laurie ;
Kaufman, Joel D. .
CIRCULATION, 2010, 121 (21) :2331-2378
[3]   Ambient particulate pollutants in the ultrafine range promote early atherosclerosis and systemic oxidative stress [J].
Araujo, Jesus A. ;
Barajas, Berenice ;
Kleinman, Michael ;
Wang, Xuping ;
Bennett, Brian J. ;
Gong, Ke Wei ;
Navab, Mohamad ;
Harkema, Jack ;
Sioutas, Constantinos ;
Lusis, Aldons J. ;
Nel, Andre E. .
CIRCULATION RESEARCH, 2008, 102 (05) :589-596
[4]   Comparability of Portable Nanoparticle Exposure Monitors [J].
Asbach, Christof ;
Kaminski, Heinz ;
Von Barany, Daniel ;
Kuhlbusch, Thomas A. J. ;
Monz, Christian ;
Dziurowitz, Nico ;
Pelzer, Johannes ;
Vossen, Katja ;
Berlin, Knut ;
Dietrich, Silvio ;
Goetz, Uwe ;
Kiesling, Heinz-Juergen ;
Schierl, Rudolf ;
Dahmann, Dirk .
ANNALS OF OCCUPATIONAL HYGIENE, 2012, 56 (05) :606-621
[5]   Effects of long-term exposure to air pollution on natural-cause mortality: an analysis of 22 European cohorts within the multicentre ESCAPE project [J].
Beelen, Rob ;
Raaschou-Nielsen, Ole ;
Stafoggia, Massimo ;
Andersen, Zorana Jovanovic ;
Weinmayr, Gudrun ;
Hoffmann, Barbara ;
Wolf, Kathrin ;
Samoli, Evangelia ;
Fischer, Paul ;
Nieuwenhuijsen, Mark ;
Vineis, Paolo ;
Xun, Wei W. ;
Katsouyanni, Klea ;
Dimakopoulou, Konstantina ;
Oudin, Anna ;
Forsberg, Bertil ;
Modig, Lars ;
Havulinna, Aki S. ;
Lanki, Timo ;
Turunen, Anu ;
Oftedal, Bente ;
Nystad, Wenche ;
Nafstad, Per ;
De Faire, Ulf ;
Pedersen, Nancy L. ;
Ostenson, Claes-Goeran ;
Fratiglioni, Laura ;
Penell, Johanna ;
Korek, Michal ;
Pershagen, Goeran ;
Eriksen, Kirsten Thorup ;
Overvad, Kim ;
Ellermann, Thomas ;
Eeftens, Marloes ;
Peeters, Petra H. ;
Meliefste, Kees ;
Wang, Meng ;
Bueno-de-Mesquita, Bas ;
Sugiri, Dorothea ;
Kraemer, Ursula ;
Heinrich, Joachim ;
de Hoogh, Kees ;
Key, Timothy ;
Peters, Annette ;
Hampel, Regina ;
Concin, Hans ;
Nagel, Gabriele ;
Ineichen, Alex ;
Schaffner, Emmanuel ;
Probst-Hensch, Nicole .
LANCET, 2014, 383 (9919) :785-795
[6]   Contribution of various microenvironments to the daily personal exposure to ultrafine particles: Personal monitoring coupled with GPS tracking [J].
Beko, Gabriel ;
Kjeldsen, Birthe Uldahl ;
Olsen, Yulia ;
Schipperijn, Jasper ;
Wierzbicka, Aneta ;
Karottki, Donna Gabriela ;
Toftum, Jorn ;
Loft, Steffen ;
Clausen, Geo .
ATMOSPHERIC ENVIRONMENT, 2015, 110 :122-129
[7]   Personal exposure to ultrafine particles: The influence of time-activity patterns [J].
Buonanno, G. ;
Stabile, L. ;
Morawska, L. .
SCIENCE OF THE TOTAL ENVIRONMENT, 2014, 468 :903-907
[8]   Early life exposure to traffic-related air pollution and allergic rhinitis in preschool children [J].
Deng, Qihong ;
Lu, Chan ;
Yu, Yichen ;
Li, Yuguo ;
Sundell, Jan ;
Norback, Dan .
RESPIRATORY MEDICINE, 2016, 121 :67-73
[9]   Active transport between home and school assessed with GPS: a cross-sectional study among Dutch elementary school children [J].
Dessing, Dirk ;
de Vries, Sanne I. ;
Graham, Jamie M. A. ;
Pierik, Frank H. .
BMC PUBLIC HEALTH, 2014, 14
[10]   Indoor and Outdoor Particle Number and Mass Concentrations in Athens. Sources, Sinks and Variability of Aerosol Parameters [J].
Diapouli, Evangelia ;
Eleftheriadis, Konstantinos ;
Karanasiou, Angeliki A. ;
Vratolis, Sterios ;
Hermansen, Ove ;
Colbeck, Ian ;
Lazaridis, Mihalis .
AEROSOL AND AIR QUALITY RESEARCH, 2011, 11 (06) :632-642