Heat integration of phenols and ammonia recovery process for the treatment of coal gasification wastewater

被引:42
作者
Gai, Hengjun [1 ]
Feng, Yirong [1 ]
Lin, Kaiqiang [1 ]
Guo, Kai [1 ]
Xiao, Meng [1 ]
Song, Hongbing [1 ]
Chen, Xiaolu [1 ]
Zhou, Hua [2 ]
机构
[1] Qingdao Univ Sci & Technol, Coll Chem Engn, Qingdao 266042, Peoples R China
[2] Cornell Univ, Chem & Biomol Engn Dept, 120 Olin Hall, Ithaca, NY 14853 USA
关键词
Phenol and ammonia recovery; Coal gasification wastewater; Heat integration; Energy conservation; Process development; CONCEPTUAL DESIGN; DISTILLATION; SIMULATION; REMOVAL; ENERGY; PLANT;
D O I
10.1016/j.cej.2017.06.033
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Coal gasification wastewater with high concentration of phenols and ammonia is difficult to biodegrade. Phenols and ammonia recovery process consisting of the sour water stripper, extraction and the solvent recovery system is applied to removing these pollutants. An improved phenol and ammonia recovery process that the sour water stripper and the solvent recovery system are thermal integrated is proposed based on the conventional wastewater treatment process. Therein, the ammonia-rich gas drawn from the middle of sour water stripper, as a heat source, is exchanged with the reboiler of the solvent distillation column and the solvent stripper. The results show that the operating cost is about 34% less than that of the conventional process, and the TAC can be decreased by about 30.8%. The proposed process of phenols and ammonia recovery for the coal gasification wastewater is proven to be an effective and economical process with a good application prospect. (C) 2017 Published by Elsevier B.V.
引用
收藏
页码:1093 / 1101
页数:9
相关论文
共 23 条
[1]   Temperature-enthalpy curve for energy targeting of distillation columns [J].
Bandyopadhyay, S ;
Malik, RK ;
Shenoy, UV .
COMPUTERS & CHEMICAL ENGINEERING, 1998, 22 (12) :1733-1744
[2]   Integrated treatment processes for coal-gasification wastewater with high concentration of phenol and ammonia [J].
Cui, Peizhe ;
Mai, Zihao ;
Yang, Siyu ;
Qian, Yu .
JOURNAL OF CLEANER PRODUCTION, 2017, 142 :2218-2226
[3]   Novel Single Stripper with Side-Draw to Remove Ammonia and Sour Gas Simultaneously for Coal-Gasification Wastewater Treatment and the Industrial Implementation [J].
Feng, Dachun ;
Yu, Zhenjiang ;
Chen, Yun ;
Qian, Yu .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2009, 48 (12) :5816-5823
[4]  
Fu G., 2012, SINOGLOBAL ENERGY, V17, P74
[5]   Optimization of existing heat-integrated refinery distillation systems [J].
Gadalla, M ;
Jobson, M ;
Smith, R .
CHEMICAL ENGINEERING RESEARCH & DESIGN, 2003, 81 (A1) :147-152
[6]   Conceptual design and retrofitting of the coal-gasification wastewater treatment process [J].
Gai, Hengjun ;
Jiang, Yanbin ;
Qian, Yu ;
Kraslawski, Andrzej .
CHEMICAL ENGINEERING JOURNAL, 2008, 138 (1-3) :84-94
[7]   Conceptual design of a modified phenol and ammonia recovery process for the treatment of coal gasification wastewater [J].
Gai, Hengjun ;
Song, Hongbing ;
Xiao, Meng ;
Feng, Yirong ;
Wu, Yumin ;
Zhou, Hua ;
Chen, Binghui .
CHEMICAL ENGINEERING JOURNAL, 2016, 304 :621-628
[8]   Industrial-scale Fixed-bed Coal Gasification: Modeling, Simulation and Thermodynamic Analysis [J].
He Chang ;
Feng Xiao ;
Chu, Khim Hoong ;
Li Anxue ;
Liu Yongjian .
CHINESE JOURNAL OF CHEMICAL ENGINEERING, 2014, 22 (05) :522-530
[9]   A review on the coal gasification wastewater treatment technologies: past, present and future outlook [J].
Ji, Qinhong ;
Tabassum, Salma ;
Hena, Sufia ;
Silva, Claudia G. ;
Yu, Guangxin ;
Zhang, Zhenjia .
JOURNAL OF CLEANER PRODUCTION, 2016, 126 :38-55
[10]   Dynamic simulation of the sour water stripping process and modified structure for effective pressure control [J].
Lee, D ;
Lee, JM ;
Lee, SY ;
Lee, IB .
CHEMICAL ENGINEERING RESEARCH & DESIGN, 2002, 80 (A2) :167-177