Self-Powered Electrostatic Filter with Enhanced Photocatalytic Degradation of Formaldehyde Based on Built-in Triboelectric Nanogenerators

被引:183
作者
Feng, Yawei [1 ,2 ]
Ling, Lili [1 ,2 ]
Nie, Jinhui [3 ]
Han, Kai [3 ]
Chen, Xiangyu [3 ]
Bian, Zhenfeng [1 ,2 ]
Li, Hexing [1 ,2 ]
Wang, Zhong Lin [3 ,4 ]
机构
[1] Shanghai Normal Univ, Educ Minist, Key & Int Joint Lab Resource Chem, Shanghai 200234, Peoples R China
[2] Shanghai Normal Univ, Shanghai Key Lab Rare Earth Funct Mat, Shanghai 200234, Peoples R China
[3] Chinese Acad Sci, Beijing Inst Nanoenergy & Nanosyst, Beijing 100083, Peoples R China
[4] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA
基金
中国国家自然科学基金;
关键词
triboelectric generator; electrostatic adsorption; photocatalysis; formaldehyde degradation; air filter; HIGHLY EFFICIENT; ENERGY; EMISSIONS; NANOFIBER;
D O I
10.1021/acsnano.7b06451
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Recently, atmospheric pollution caused by particulate matter or volatile organic compounds (VOCs) has become a serious issue to threaten human health. Consequently, it is highly desirable to develop an efficient purifying technique with simple structure and low cost. In this study, by combining a triboelectric nanogenerator (TENG) and a photocatalysis technique, we demonstrated a concept of a self-powered filtering method for removing pollutants from indoor atmosphere. The photocatalyst P25 or Pt/P25 was embedded on the surface of polymer-coated stainless steel wires, and such steel wires were woven into a filtering network. A strong electric field can be induced on this filtering network by TENG, while both electrostatic adsorption effect and TENG-enhanced photocatalytic effect can be achieved. Rhodamine B (RhB) steam was selected as the pollutant for demonstration. The absorbed RhB on the filter network with TENG in 1 min was almost the same amount of absorption achieved in 15 min without using TENG. Meanwhile, the degradation of RhB was increased over 50% under the drive of TENG. Furthermore, such a device was applied for the degradation of formaldehyde, where degradation efficiency was doubled under the drive of TENG. This work extended the application for the TENG in self-powered electrochemistry, design and concept of which can be possibly applied in the field of haze governance, indoor air cleaning, and photocatalytic pollution removal for environmental protection.
引用
收藏
页码:12411 / 12418
页数:8
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