Self-Powered Electrostatic Filter with Enhanced Photocatalytic Degradation of Formaldehyde Based on Built-in Triboelectric Nanogenerators

被引:188
作者
Feng, Yawei [1 ,2 ]
Ling, Lili [1 ,2 ]
Nie, Jinhui [3 ]
Han, Kai [3 ]
Chen, Xiangyu [3 ]
Bian, Zhenfeng [1 ,2 ]
Li, Hexing [1 ,2 ]
Wang, Zhong Lin [3 ,4 ]
机构
[1] Shanghai Normal Univ, Educ Minist, Key & Int Joint Lab Resource Chem, Shanghai 200234, Peoples R China
[2] Shanghai Normal Univ, Shanghai Key Lab Rare Earth Funct Mat, Shanghai 200234, Peoples R China
[3] Chinese Acad Sci, Beijing Inst Nanoenergy & Nanosyst, Beijing 100083, Peoples R China
[4] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA
基金
中国国家自然科学基金;
关键词
triboelectric generator; electrostatic adsorption; photocatalysis; formaldehyde degradation; air filter; HIGHLY EFFICIENT; ENERGY; EMISSIONS; NANOFIBER;
D O I
10.1021/acsnano.7b06451
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Recently, atmospheric pollution caused by particulate matter or volatile organic compounds (VOCs) has become a serious issue to threaten human health. Consequently, it is highly desirable to develop an efficient purifying technique with simple structure and low cost. In this study, by combining a triboelectric nanogenerator (TENG) and a photocatalysis technique, we demonstrated a concept of a self-powered filtering method for removing pollutants from indoor atmosphere. The photocatalyst P25 or Pt/P25 was embedded on the surface of polymer-coated stainless steel wires, and such steel wires were woven into a filtering network. A strong electric field can be induced on this filtering network by TENG, while both electrostatic adsorption effect and TENG-enhanced photocatalytic effect can be achieved. Rhodamine B (RhB) steam was selected as the pollutant for demonstration. The absorbed RhB on the filter network with TENG in 1 min was almost the same amount of absorption achieved in 15 min without using TENG. Meanwhile, the degradation of RhB was increased over 50% under the drive of TENG. Furthermore, such a device was applied for the degradation of formaldehyde, where degradation efficiency was doubled under the drive of TENG. This work extended the application for the TENG in self-powered electrochemistry, design and concept of which can be possibly applied in the field of haze governance, indoor air cleaning, and photocatalytic pollution removal for environmental protection.
引用
收藏
页码:12411 / 12418
页数:8
相关论文
共 31 条
[1]   Impacts and mitigation of excess diesel-related NOx emissions in 11 major vehicle markets [J].
Anenberg, Susan C. ;
Miller, Joshua ;
Injares, Ray M. ;
Du, Li ;
Henze, Daven K. ;
Lacey, Forrest ;
Malley, Christopher S. ;
Emberson, Lisa ;
Franco, Vicente ;
Klimont, Zbigniew ;
Heyes, Chris .
NATURE, 2017, 545 (7655) :467-+
[2]   Formaldehyde removal by common indoor plant species and various growing media [J].
Aydogan, Ahu ;
Montoya, Lupita D. .
ATMOSPHERIC ENVIRONMENT, 2011, 45 (16) :2675-2682
[3]   Self-powered cleaning of air pollution by wind driven triboelectric nanogenerator [J].
Chen, Shuwen ;
Gao, Caizhen ;
Tang, Wei ;
Zhu, Huarui ;
Han, Yu ;
Jiang, Qianwen ;
Li, Tao ;
Cao, Xia ;
Wang, Zhonglin .
NANO ENERGY, 2015, 14 :217-225
[4]   Self-powered modulation of elastomeric optical grating by using triboelectric nanogenerator [J].
Chen, Xiangyu ;
Wu, Yali ;
Yu, Aifang ;
Xu, Liang ;
Zheng, Li ;
Liu, Yongsheng ;
Li, Hexing ;
Wang, Zhong Lin .
NANO ENERGY, 2017, 38 :91-100
[5]   Tunable Optical Modulator by Coupling a Triboelectric Nanogenerator and a Dielectric Elastomer [J].
Chen, Xiangyu ;
Pu, Xiong ;
Jiang, Tao ;
Yu, Aifang ;
Xu, Liang ;
Wang, Zhong Lin .
ADVANCED FUNCTIONAL MATERIALS, 2017, 27 (01)
[6]   Spontaneous electrical charging of droplets by conventional pipetting [J].
Choi, Dongwhi ;
Lee, Horim ;
Im, Do Jin ;
Kang, In Seok ;
Lim, Geunbae ;
Kim, Dong Sung ;
Kang, Kwan Hyoung .
SCIENTIFIC REPORTS, 2013, 3
[7]   High performance sound driven triboelectric nanogenerator for harvesting noise energy [J].
Cui, Nuanyang ;
Gu, Long ;
Liu, Jinmei ;
Bai, Suo ;
Qiu, Jiawen ;
Fu, Jiecai ;
Kou, Xinli ;
Liu, Hong ;
Qin, Yong ;
Wang, Zhong Lin .
NANO ENERGY, 2015, 15 :321-328
[8]   Effect of Ferroelectricity on Solar-Light-Driven Photocatalytic Activity of BaTiO3-Influence on the Carrier Separation and Stern Layer Formation [J].
Cui, Yongfei ;
Briscoe, Joe ;
Dunn, Steve .
CHEMISTRY OF MATERIALS, 2013, 25 (21) :4215-4223
[9]   Flexible triboelectric generator! [J].
Fan, Feng-Ru ;
Tian, Zhong-Qun ;
Wang, Zhong Lin .
NANO ENERGY, 2012, 1 (02) :328-334
[10]   Transparent Triboelectric Nanogenerators and Self-Powered Pressure Sensors Based on Micropatterned Plastic Films [J].
Fan, Feng-Ru ;
Lin, Long ;
Zhu, Guang ;
Wu, Wenzhuo ;
Zhang, Rui ;
Wang, Zhong Lin .
NANO LETTERS, 2012, 12 (06) :3109-3114