Process systems engineering studies for the synthesis of catalytic biomass-to-fuels strategies

被引:46
作者
Han, Jeehoon [1 ]
Sen, S. Murat [1 ]
Luterbacher, Jeremy S. [1 ]
Alonso, David Martin [1 ]
Dumesic, James A. [1 ]
Maravelias, Christos T. [1 ]
机构
[1] Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 53706 USA
关键词
Lignocellulosic biofuels; Process synthesis; Technoeconomic evaluation; Heterogeneous catalysis; NONENZYMATIC SUGAR PRODUCTION; LIQUID-HYDROCARBON FUELS; TECHNOECONOMIC ANALYSIS; LIGNOCELLULOSIC ETHANOL; TRANSPORTATION FUELS; CORN STOVER; GAMMA-VALEROLACTONE; HYDROLYSIS PROCESS; OPTIMAL-DESIGN; SULFURIC-ACID;
D O I
10.1016/j.compchemeng.2015.04.007
中图分类号
TP39 [计算机的应用];
学科分类号
081203 ; 0835 ;
摘要
The goal of this paper is to show how chemical process synthesis and analysis studies can be coupled with experimental heterogeneous catalysis studies to identify promising research directions for the development of strategies for the production of renewable fuels. We study five catalytic biomass-to-fuels strategies that rely on production of platform chemicals, such as levulinic acid and fermentable sugars. We first integrate catalytic conversion subsystems with separation subsystems to generate complete conversion strategies, and we then develop the corresponding process simulation models based on experimental results. Our analyses suggest that catalytic biomass-to-fuel conversion strategies could become economically competitive alternatives to current biofuel production approaches as a result of iterative experimental and computational efforts. (c) 2015 Elsevier Ltd. All rights reserved.
引用
收藏
页码:57 / 69
页数:13
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