Herein, the heavy metal removal efficiency of Philippine natural zeolite is investigated through a comparative study with commercial alumina (Al2O3). XRD results revealed a high purity crystalline gamma-Al2O3 and a natural zeolite having clinoptilolite (Na,K,Ca)(2-3)Al-3(Al,Si)(2)Si13O36 center dot 12H(2)O and mordenite (Ca, Na-2, K-2)Al2Si10O24 center dot 7H(2)O as primary component minerals. Micro-pores and plate-like structures were observed on the surface of the natural zeolite. The natural zeolite has shown three times higher removal efficiency for Zn2+ ion than alumina. On the other hand, alumina exhibited comparable but smaller removal efficiency for As3+ as with that of natural zeolite. Alumina showed a higher capability of increasing the pH of both solutions compared with the natural zeolite. Based on removal efficiency and adsorbent costs, Philippine natural zeolite could be used as a low-cost alternative for wastewater treatment.