The LXCat project: Electron scattering cross sections and swarm parameters for low temperature plasma modeling

被引:225
作者
Pancheshnyi, S. [1 ,2 ]
Biagi, S. [3 ]
Bordage, M. C. [1 ,2 ]
Hagelaar, G. J. M. [1 ,2 ]
Morgan, W. L. [4 ]
Phelps, A. V. [5 ,6 ]
Pitchford, L. C. [1 ,2 ]
机构
[1] Univ Toulouse, UPS, INPT, LAPLACE Lab Plasma & Convers Energie, F-31062 Toulouse 9, France
[2] CNRS, LAPLACE, F-31062 Toulouse, France
[3] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 7ZE, Merseyside, England
[4] Kinema Res & Software, Monument, CO 80132 USA
[5] NIST, JILA, Boulder, CO 80309 USA
[6] Univ Colorado, Boulder, CO 80309 USA
关键词
Low temperature plasma modeling; On-line databases; Electron-neutral cross sections; Electron swarm parameters; Boltzmann calculation; FOURIER-TRANSFORM SPECTROSCOPY; IMPACT EXCITATION; TRANSPORT COEFFICIENTS; BOLTZMANN-EQUATION; ARGON; IONIZATION; COLLISIONS; DISCHARGE; RATIOS; VALUES;
D O I
10.1016/j.chemphys.2011.04.020
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
LXCat is a dynamic, open-access, website for collecting, displaying, and downloading ELECtron SCATtering cross sections and swarm parameters (mobility, diffusion coefficient, reaction rates, etc.) required for modeling low temperature, non-equilibrium plasmas. Contributors set up individual databases, and the available databases, indicated by the contributor's chosen title, include mainly complete sets of electron-neutral scattering cross sections, although the option for introducing partial sets of cross sections exists. A database for measured swarm parameters is also part of LXCat, and this is a growing activity. On-line tools include options for browsing, plotting, and downloading cross section data. The electron energy distribution functions (edfs) in low temperature plasmas are in general non-Maxwellian, and LXCat provides an option for execution of an on-line Boltzmann equation solver to calculate the edf in homogeneous electric fields. Thus, the user can obtain electron transport and rate coefficients (averages over the edfs) in pure gases or gas mixtures over a range of values of the reduced electric fields strength, E/N, the ratio of the electric field strength to the neutral density, using cross sections from the available databases. New contributors are welcome and anyone wishing to create a database and upload data can request a username and password. LXCat is part of a larger, community-wide effort aimed at collecting, evaluating, and sharing data relevant to modeling low temperature plasmas. To illustrate the utility of LXCat in this context, we compare electron swarm parameters in argon calculated using the different compilations of cross sections presently available on LXCat. These compilations include quite different groupings of excited states, yet lead to swarm parameters in good agreement. LXCat is available at http://www.lxcat.laplace.univ-tlse.fr. (C) 2011 Elsevier B. V. All rights reserved.
引用
收藏
页码:148 / 153
页数:6
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