Molecular alignment dependent electron interference in attosecond ultraviolet photoionization

被引:11
作者
Yuan, Kai-Jun [1 ]
Bandrauk, Andre D. [1 ]
机构
[1] Univ Sherbrooke, Fac Sci, Chim Theor Lab, Sherbrooke, PQ J1K 2R1, Canada
来源
STRUCTURAL DYNAMICS-US | 2015年 / 2卷 / 01期
基金
加拿大自然科学与工程研究理事会;
关键词
LASER; IONIZATION; DIFFRACTION; DYNAMICS; FIELD;
D O I
10.1063/1.4906126
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We present molecular photoionization processes by intense attosecond ultraviolet laser pulses from numerical solutions of time-dependent Schrodinger equations. Simulations preformed on a single electron diatomic H-2(+) show minima in molecular photoelectron energy spectra resulting from two center interference effects which depend strongly on molecular alignment. We attribute such sensitivity to the spatial orientation asymmetry of the photoionization process from the two nuclei. A similar influence on photoelectron kinetic energies is also presented. (C) 2015 Author(s).
引用
收藏
页数:9
相关论文
共 50 条
  • [41] Visualization and interpretation of attosecond electron dynamics in laser-driven hydrogen molecular ion using Bohmian trajectories
    Takemoto, Norio
    Becker, Andreas
    JOURNAL OF CHEMICAL PHYSICS, 2011, 134 (07)
  • [42] Photoionization of resonantly driven atomic states by an extreme ultraviolet-free-electron laser: intensity dependence and renormalization of Rabi frequencies
    Kaiser, B.
    Brand, A.
    Glaessl, M.
    Vagov, A.
    Axt, V. M.
    Pietsch, U.
    NEW JOURNAL OF PHYSICS, 2013, 15
  • [43] Interference between Molecular and Photon Field-Mediated Electron Transfer in Cavities
    Chowdhury, Sutirtha N.
    Zhang, Peng
    Beratan, David N.
    JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 2022, 13 (42) : 9822 - 9828
  • [44] In-situ analysis of volatile products from lignite pyrolysis with pyrolysis-vacuum ultraviolet photoionization and electron impact mass spectrometry
    Li, Gang
    Zhang, Shi-Yu
    Jin, Li-Jun
    Tang, Zi-Chao
    Hu, Hao-Quan
    FUEL PROCESSING TECHNOLOGY, 2015, 133 : 232 - 236
  • [45] Catalytic decomposition of methane on impregnated nickel based anodes with molecular-beam mass spectrometry and tunable synchrotron vacuum ultraviolet photoionization
    Liu, Beibei
    Liu, Zhangbo
    Wang, Shuang
    Xia, Changrong
    Xie, Mingfeng
    Cheng, Zhanjun
    Li, Yuyang
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2012, 37 (10) : 8354 - 8359
  • [46] Probing combustion and catalysis intermediates by synchrotron vacuum ultraviolet photoionization molecular-beam mass spectrometry: recent progress and future opportunities
    Zhou, Zhongyue
    Yang, Jiuzhong
    Yuan, Wenhao
    Wang, Zhandong
    Pan, Yang
    Qi, Fei
    PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2022, 24 (36) : 21567 - 21577
  • [47] Electron vacancy-level dependent hybrid photoionization of the F- @C60+ molecule: a novel effect
    Ali, Esam
    O'Brien, Taylor
    Dennis, Andrew
    Madjet, Mohamed El-Amine
    Manson, Steven T.
    Chakraborty, Himadri S.
    JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 2022, 55 (04)
  • [48] Effect of low-energy electron interference on strong-field molecular ionization
    Hu, Shilin
    Chen, Jing
    Hao, Xiaolei
    Li, Weidong
    PHYSICAL REVIEW A, 2016, 93 (02)
  • [49] Electron-nuclear entanglement in the time-dependent molecular wavefunction
    Agostini, Federica
    Gross, E. K. U.
    Curchod, Basile F. E.
    COMPUTATIONAL AND THEORETICAL CHEMISTRY, 2019, 1151 : 99 - 106
  • [50] Nonadiabatic Molecular Dynamics of Water Cluster Dissociation by Vacuum Ultraviolet Absorption or Electron Impact Excitation
    Jones, Leighton O.
    Schatz, George C.
    JOURNAL OF PHYSICAL CHEMISTRY B, 2024, 128 (12) : 2948 - 2954