Investigation of Optical Properties of Ceramic Ce:GAGG by High Temperature Annealing

被引:10
作者
Park, Chansun [1 ]
Ullah, Muhammad Nasir [1 ]
Kim, Chanho [1 ]
Cho, Shinhaeng [2 ]
Yeom, Jung-Yeol [1 ,3 ]
机构
[1] Korea Univ, Dept Bioconvergence Engn, Seoul 02841, South Korea
[2] Chonnam Natl Univ, Med Sch, Gwangju 61186, South Korea
[3] Korea Univ, Sch Biomed Engn, Seoul 02841, South Korea
基金
新加坡国家研究基金会;
关键词
Scintillator; Light output; Energy resolution; Gamma-rays; X-ray Photoelectron Spectroscopy; SCINTILLATORS; DEFECTS;
D O I
10.3938/jkps.75.962
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
An as-fabricated cerium-doped ceramic scintillator Gd3Al2Ga3O12 (Ce:GAGG) was thermally annealed at different temperatures. The light output and energy resolution of the scintillators were measured before and after thermal treatment. The effect of thermal annealing in the air at high temperature (at 1000 degrees C for 5 hours) deforms the microstructure by mitigating oxygen vacancies of the ceramic scintillator. This has been proven by XPS study that showed the existence of oxygen vacancies and subsequent decrease of oxygen deficiency amid annealing treatment that led to an output signal increase. The diffusion ability of oxygen atoms by annealing played a key role in compensating for defect sites. In this study, by controlling thermodynamic conditions, the light output was enhanced by similar to 30.4% and the energy resolution improved by similar to 2.4% after annealing at 1000 degrees C in the air.
引用
收藏
页码:962 / 967
页数:6
相关论文
共 26 条
[1]   SPECTROSCOPY AND SCINTILLATION PROPERTIES OF CERIUM-DOPED YALO3 SINGLE-CRYSTALS [J].
BARYSHEVSKY, VG ;
KORZHIK, MV ;
MINKOV, BI ;
SMIRNOVA, SA ;
FYODOROV, AA ;
DORENBOS, P ;
VANEIJK, CWE .
JOURNAL OF PHYSICS-CONDENSED MATTER, 1993, 5 (42) :7893-7902
[2]   Defects Identification and Effects of Annealing on Lu2(1-x)Y2xSiO5 (LYSO) Single Crystals for Scintillation Application [J].
Blahuta, Samuel ;
Bessiere, Aurelie ;
Viana, Bruno ;
Ouspenski, Vladimir ;
Mattmann, Eric ;
Lejay, Julien ;
Gourier, Didier .
MATERIALS, 2011, 4 (07) :1224-1237
[3]  
Carel W., 2002, PHYS MED BIOL, V47, P85
[4]   Transparent Ceramic Scintillators for Gamma Spectroscopy and Radiography [J].
Cherepy, N. J. ;
Kuntz, J. D. ;
Seeley, Z. M. ;
Fisher, S. E. ;
Drury, O. B. ;
Sturm, B. W. ;
Hurst, T. A. ;
Sanner, R. D. ;
Roberts, J. J. ;
Payne, S. A. .
HARD X-RAY, GAMMA-RAY, AND NEUTRON DETECTOR PHYSICS XII, 2010, 7805
[5]   Air Atmosphere Annealing Effects on LSO:Ce Crystal [J].
Ding, Dongzhou ;
Feng, He ;
Ren, Guohao ;
Nikl, Martin ;
Qin, Laishun ;
Pan, Shangke ;
Yang, Fan .
IEEE TRANSACTIONS ON NUCLEAR SCIENCE, 2010, 57 (03) :1272-1277
[6]   Effect of thermal annealing on light yield, low temperature thermoluminescence, and time profiles of LuAG:Pr scintillator crystals [J].
Drozdowski, Winicjusz ;
Brylew, Kamil ;
Witkowski, Marcin E. ;
Wojtowicz, Andrzej J. ;
Kamada, Kei ;
Yanagida, Takayuki ;
Yoshikawa, Akira .
RADIATION MEASUREMENTS, 2013, 56 :80-83
[7]   Ceramic scintillators [J].
Greskovich, C ;
Duclos, S .
ANNUAL REVIEW OF MATERIALS SCIENCE, 1997, 27 :69-88
[8]  
Humphreys F. J., 2012, RECRYSTALLIZATION RE, P4
[9]   Characteristics of a nonstoichiometric Gd3+δ(Al,Ga)5-δO12:Ce garnet scintillator [J].
Kanai, Tsuneyuki ;
Satoh, Makoto ;
Miura, Ichiro .
JOURNAL OF THE AMERICAN CERAMIC SOCIETY, 2008, 91 (02) :456-462
[10]   A new lutetia-based ceramic scintillator for X-ray imaging [J].
Lempicki, A ;
Brecher, C ;
Szupryczynski, P ;
Lingertat, H ;
Nagarkar, VV ;
Tipnis, SV ;
Miller, SR .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT, 2002, 488 (03) :579-590