Global fine-scale changes in ambient NO2 during COVID-19 lockdowns

被引:154
作者
Cooper, Matthew J. [1 ,2 ]
Martin, Randall, V [1 ,2 ,3 ]
Hammer, Melanie S. [1 ,2 ]
Levelt, Pieternel F. [4 ,5 ,6 ]
Veefkind, Pepijn [4 ,7 ]
Lamsal, Lok N. [8 ,9 ]
Krotkov, Nickolay A. [8 ]
Brook, Jeffrey R. [10 ,11 ]
McLinden, Chris A. [12 ]
机构
[1] Dalhousie Univ, Dept Phys & Atmospher Sci, Halifax, NS, Canada
[2] Washington Univ, Dept Energy Environm & Chem Engn, St Louis, MO 63110 USA
[3] Harvard Smithsonian Ctr Astrophys, 60 Garden St, Cambridge, MA 02138 USA
[4] Royal Netherlands Meteorol Inst KNMI, De Bilt, Netherlands
[5] Univ Technol Delft, Delft, Netherlands
[6] Natl Ctr Atmospher Res, POB 3000, Boulder, CO 80307 USA
[7] Delft Univ Technol, Dept Geosci & Remote Sensing, Delft, Netherlands
[8] NASA, Goddard Space Flight Ctr, Greenbelt, MD USA
[9] Univ Space Res Assoc, Columbia, MD USA
[10] Univ Toronto, Dalla Lana Sch Publ Hlth, Toronto, ON, Canada
[11] Univ Toronto, Dept Chem Engn & Appl Chem, Toronto, ON, Canada
[12] Environm & Climate Change Canada, Toronto, ON, Canada
关键词
NITROGEN-DIOXIDE; TROPOSPHERIC NO2; AIR-QUALITY; S5P TROPOMI; TRENDS; SURFACE; POLLUTION; SATELLITE; SPACE; METEOROLOGY;
D O I
10.1038/s41586-021-04229-0
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Nitrogen dioxide (NO2) is an important contributor to air pollution and can adversely affect human health(1-9). A decrease in NO2 concentrations has been reported as a result of lockdown measures to reduce the spread of COVID-19(10-20). Questions remain, however, regarding the relationship of satellite-derived atmospheric column NO2 data with health-relevant ambient ground-level concentrations, and the representativeness of limited ground-based monitoring data for global assessment. Here we derive spatially resolved, global ground-level NO2 concentrations from NO2 column densities observed by the TROPOMI satellite instrument at sufficiently fine resolution (approximately one kilometre) to allow assessment of individual cities during COVID-19 lockdowns in 2020 compared to 2019. We apply these estimates to quantify NO2 changes in more than 200 cities, including 65 cities without available ground monitoring, largely in lower-income regions. Mean country-level population-weighted NO2 concentrations are 29% +/- 3% lower in countries with strict lockdown conditions than in those without. Relative to long-term trends, NO2 decreases during COVID-19 lockdowns exceed recent Ozone Monitoring Instrument (OMI)-derived year-to-year decreases from emission controls, comparable to 15 +/- 4 years of reductions globally. Our case studies indicate that the sensitivity of NO2 to lockdowns varies by country and emissions sector, demonstrating the critical need for spatially resolved observational information provided by these satellite-derived surface concentration estimates.
引用
收藏
页码:380 / +
页数:11
相关论文
共 70 条
[31]   Lung Cancer and Exposure to Nitrogen Dioxide and Traffic: A Systematic Review and Meta-Analysis [J].
Hamra, Ghassan B. ;
Laden, Francine ;
Cohen, Aaron J. ;
Raaschou-Nielsen, Ole ;
Brauer, Michael ;
Loomis, Dana .
ENVIRONMENTAL HEALTH PERSPECTIVES, 2015, 123 (11) :1107-1112
[32]  
Hilboll A., 2017, ATMOS CHEM PHYS, V35, P703, DOI [10.5194/acp-2017-101, DOI 10.5194/ACP-2017-101]
[33]   Evaluating the impact of spatial resolution on tropospheric NO2 column comparisons within urban areas using high-resolution airborne data [J].
Judd, Laura M. ;
Al-Saadi, Jassim A. ;
Janz, Scott J. ;
Kowalewski, Matthew G. ;
Pierce, R. Bradley ;
Szykman, James J. ;
Valin, Lukas C. ;
Swap, Robert ;
Cede, Alexander ;
Mueller, Moritz ;
Tiefengraber, Martin ;
Abuhassan, Nader ;
Williams, David .
ATMOSPHERIC MEASUREMENT TECHNIQUES, 2019, 12 (11) :6091-6111
[34]   Global impact of COVID-19 restrictions on the surface concentrations of nitrogen dioxide and ozone [J].
Keller, Christoph A. ;
Evans, Mathew J. ;
Knowland, K. Emma ;
Hasenkopf, Christa A. ;
Modekurty, Sruti ;
Lucchesi, Robert A. ;
Oda, Tomohiro ;
Franca, Bruno B. ;
Mandarino, Felipe C. ;
Diaz Suarez, M. Valeria ;
Ryan, Robert G. ;
Fakes, Luke H. ;
Pawson, Steven .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2021, 21 (05) :3555-3592
[35]   COVID-19 pandemic reveals persistent disparities in nitrogen dioxide pollution [J].
Kerr, Gaige Hunter ;
Goldberg, Daniel L. ;
Anenberg, Susan C. .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2021, 118 (30)
[36]   Assessment of the magnitude and recent trends in satellite-derived ground-level nitrogen dioxide over North America [J].
Kharol, S. K. ;
Martin, R. V. ;
Philip, S. ;
Boys, B. ;
Lamsal, L. N. ;
Jerrett, M. ;
Brauer, M. ;
Crouse, D. L. ;
McLinden, C. ;
Burnett, R. T. .
ATMOSPHERIC ENVIRONMENT, 2015, 118 :236-245
[37]   Sudden changes in nitrogen dioxide emissions over Greece due to lockdown after the outbreak of COVID-19 [J].
Koukouli, Maria-Elissavet ;
Skoulidou, Ioanna ;
Karavias, Andreas ;
Parcharidis, Isaak ;
Balis, Dimitris ;
Manders, Astrid ;
Segers, Arjo ;
Eskes, Henk ;
van Geffen, Jos .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2021, 21 (03) :1759-1774
[38]   Aura OMI observations of regional SO2 and NO2 pollution changes from 2005 to 2015 [J].
Krotkov, Nickolay A. ;
McLinden, Chris A. ;
Li, Can ;
Lamsal, Lok N. ;
Celarier, Edward A. ;
Marchenko, Sergey V. ;
Swartz, William H. ;
Bucsela, Eric J. ;
Joiner, Joanna ;
Duncan, Bryan N. ;
Boersma, K. Folkert ;
Veefkind, J. Pepijn ;
Levelt, Pieternel F. ;
Fioletov, Vitali E. ;
Dickerson, Russell R. ;
He, Hao ;
Lu, Zifeng ;
Streets, David G. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2016, 16 (07) :4605-4629
[39]   Ground-level nitrogen dioxide concentrations inferred from the satellite-borne Ozone Monitoring Instrument [J].
Lamsal, L. N. ;
Martin, R. V. ;
van Donkelaar, A. ;
Steinbacher, M. ;
Celarier, E. A. ;
Bucsela, E. ;
Dunlea, E. J. ;
Pinto, J. P. .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2008, 113 (D16)
[40]   Ozone Monitoring Instrument (OMI) Aura nitrogen dioxide standard product version 4.0 with improved surface and cloud treatments [J].
Lamsal, Lok N. ;
Krotkov, Nickolay A. ;
Vasilkov, Alexander ;
Marchenko, Sergey ;
Qin, Wenhan ;
Yang, Eun-Su ;
Fasnacht, Zachary ;
Joiner, Joanna ;
Choi, Sungyeon ;
Haffner, David ;
Swartz, William H. ;
Fisher, Bradford ;
Bucsela, Eric .
ATMOSPHERIC MEASUREMENT TECHNIQUES, 2021, 14 (01) :455-479