Global fine-scale changes in ambient NO2 during COVID-19 lockdowns

被引:154
作者
Cooper, Matthew J. [1 ,2 ]
Martin, Randall, V [1 ,2 ,3 ]
Hammer, Melanie S. [1 ,2 ]
Levelt, Pieternel F. [4 ,5 ,6 ]
Veefkind, Pepijn [4 ,7 ]
Lamsal, Lok N. [8 ,9 ]
Krotkov, Nickolay A. [8 ]
Brook, Jeffrey R. [10 ,11 ]
McLinden, Chris A. [12 ]
机构
[1] Dalhousie Univ, Dept Phys & Atmospher Sci, Halifax, NS, Canada
[2] Washington Univ, Dept Energy Environm & Chem Engn, St Louis, MO 63110 USA
[3] Harvard Smithsonian Ctr Astrophys, 60 Garden St, Cambridge, MA 02138 USA
[4] Royal Netherlands Meteorol Inst KNMI, De Bilt, Netherlands
[5] Univ Technol Delft, Delft, Netherlands
[6] Natl Ctr Atmospher Res, POB 3000, Boulder, CO 80307 USA
[7] Delft Univ Technol, Dept Geosci & Remote Sensing, Delft, Netherlands
[8] NASA, Goddard Space Flight Ctr, Greenbelt, MD USA
[9] Univ Space Res Assoc, Columbia, MD USA
[10] Univ Toronto, Dalla Lana Sch Publ Hlth, Toronto, ON, Canada
[11] Univ Toronto, Dept Chem Engn & Appl Chem, Toronto, ON, Canada
[12] Environm & Climate Change Canada, Toronto, ON, Canada
关键词
NITROGEN-DIOXIDE; TROPOSPHERIC NO2; AIR-QUALITY; S5P TROPOMI; TRENDS; SURFACE; POLLUTION; SATELLITE; SPACE; METEOROLOGY;
D O I
10.1038/s41586-021-04229-0
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Nitrogen dioxide (NO2) is an important contributor to air pollution and can adversely affect human health(1-9). A decrease in NO2 concentrations has been reported as a result of lockdown measures to reduce the spread of COVID-19(10-20). Questions remain, however, regarding the relationship of satellite-derived atmospheric column NO2 data with health-relevant ambient ground-level concentrations, and the representativeness of limited ground-based monitoring data for global assessment. Here we derive spatially resolved, global ground-level NO2 concentrations from NO2 column densities observed by the TROPOMI satellite instrument at sufficiently fine resolution (approximately one kilometre) to allow assessment of individual cities during COVID-19 lockdowns in 2020 compared to 2019. We apply these estimates to quantify NO2 changes in more than 200 cities, including 65 cities without available ground monitoring, largely in lower-income regions. Mean country-level population-weighted NO2 concentrations are 29% +/- 3% lower in countries with strict lockdown conditions than in those without. Relative to long-term trends, NO2 decreases during COVID-19 lockdowns exceed recent Ozone Monitoring Instrument (OMI)-derived year-to-year decreases from emission controls, comparable to 15 +/- 4 years of reductions globally. Our case studies indicate that the sensitivity of NO2 to lockdowns varies by country and emissions sector, demonstrating the critical need for spatially resolved observational information provided by these satellite-derived surface concentration estimates.
引用
收藏
页码:380 / +
页数:11
相关论文
共 70 条
[1]   Global, national, and urban burdens of paediatric asthma incidence attributable to ambient NO2 pollution: estimates from global datasets [J].
Achakulwisut, Pattanun ;
Brauer, Michael ;
Hystad, Perry ;
Anenberg, Susan C. .
LANCET PLANETARY HEALTH, 2019, 3 (04) :E166-E178
[2]  
Anenberg SC, 2018, ENVIRON HEALTH PERSP, V126, DOI [10.1289/ehp3766, 10.1289/EHP3766]
[3]   Fifteen-year trends in criteria air pollutants in oil sands communities of Alberta, Canada [J].
Bari, Md. ;
Kindzierski, Warren B. .
ENVIRONMENT INTERNATIONAL, 2015, 74 :200-208
[4]   OMI air-quality monitoring over the Middle East [J].
Barkley, Michael P. ;
Abad, Gonzalo Gonzalez ;
Kurosu, Thomas P. ;
Spurr, Robert ;
Torbatian, Sara ;
Lerot, Christophe .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2017, 17 (07) :4687-4709
[5]   Impact of Coronavirus Outbreak on NO2Pollution Assessed Using TROPOMI and OMI Observations [J].
Bauwens, M. ;
Compernolle, S. ;
Stavrakou, T. ;
Muller, J-F ;
van Gent, J. ;
Eskes, H. ;
Levelt, P. F. ;
van der A, R. ;
Veefkind, J. P. ;
Vlietinck, J. ;
Yu, H. ;
Zehner, C. .
GEOPHYSICAL RESEARCH LETTERS, 2020, 47 (11)
[6]   Analysis of Criteria Air Pollutant Trends in Three Mexican Metropolitan Areas [J].
Benitez-Garcia, Sandy-Edith ;
Kanda, Isao ;
Wakamatsu, Shinji ;
Okazaki, Yukiyo ;
Kawano, Masahide .
ATMOSPHERE, 2014, 5 (04) :806-829
[7]   Global modeling of tropospheric chemistry with assimilated meteorology: Model description and evaluation [J].
Bey, I ;
Jacob, DJ ;
Yantosca, RM ;
Logan, JA ;
Field, BD ;
Fiore, AM ;
Li, QB ;
Liu, HGY ;
Mickley, LJ ;
Schultz, MG .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2001, 106 (D19) :23073-23095
[8]   COVID-19 lockdown-induced changes in NO2 levels across India observed by multi-satellite and surface observations [J].
Biswal, Akash ;
Singh, Vikas ;
Singh, Shweta ;
Kesarkar, Amit P. ;
Ravindra, Khaiwal ;
Sokhi, Ranjeet S. ;
Chipperfield, Martyn P. ;
Dhomse, Sandip S. ;
Pope, Richard J. ;
Singh, Tanbir ;
Mor, Suman .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2021, 21 (06) :5235-5251
[9]   Improving algorithms and uncertainty estimates for satellite NO2 retrievals: results from the quality assurance for the essential climate variables (QA4ECV) project [J].
Boersma, K. Folkert ;
Eskes, Henk J. ;
Richter, Andreas ;
De Smedt, Isabelle ;
Lorente, Alba ;
Beirle, Steffen ;
van Geffen, Jos H. G. M. ;
Zara, Marina ;
Peters, Enno ;
Van Roozendael, Michel ;
Wagner, Thomas ;
Maasakkers, Joannes D. ;
van der A, Ronald J. ;
Nightingale, Joanne ;
De Rudder, Anne ;
Irie, Hitoshi ;
Pinardi, Gaia ;
Lambert, Jean-Christopher ;
Compernolle, Steven C. .
ATMOSPHERIC MEASUREMENT TECHNIQUES, 2018, 11 (12) :6651-6678
[10]   Further interpretation of the acute effect of nitrogen dioxide observed in Canadian time-series studies [J].
Brook, Jeffrey R. ;
Burnett, Richard T. ;
Dann, Tom F. ;
Cakmak, Sabit ;
Goldberg, Mark S. ;
Fan, Xinghua ;
Wheeler, Amanda J. .
JOURNAL OF EXPOSURE SCIENCE AND ENVIRONMENTAL EPIDEMIOLOGY, 2007, 17 (Suppl 2) :S36-S44