3D Ag/NiCo-layered double hydroxide with adsorptive and photocatalytic performance

被引:25
作者
Wang, Tao [1 ,3 ]
Liu, Xiqing [2 ]
Ma, Changchang [1 ,3 ]
Liu, Yang [3 ,4 ]
Dong, Hongjun [1 ,3 ]
Ma, Wei [3 ,5 ]
Liu, Zhi [3 ,6 ]
Wei, Maobin [3 ,4 ]
Li, Chunxiang [1 ,3 ]
Yan, Yongsheng [1 ,3 ]
机构
[1] Jiangsu Univ, Sch Chem & Chem Engn, Zhenjiang 212013, Peoples R China
[2] Jiangsu Univ, Sch Mat Sci & Engn, Zhenjiang 212013, Peoples R China
[3] Jiangsu Univ, Inst Green Chem & Chem Technol, Zhenjiang 212013, Peoples R China
[4] Jilin Normal Univ, Coll Phys, Siping 13600, Peoples R China
[5] Jiangsu United Chem Co Ltd, Zhenjiang 212212, Jiangsu, Peoples R China
[6] Liaoning Normal Univ, Sch Environm & Safety Engn, Dalian 116029, Peoples R China
基金
美国国家科学基金会; 中国博士后科学基金;
关键词
3D NiCo-LDHs; Ag nanoparticles; Surface plasma resonance; Adsorption performance; Photocatalytic mechanism; CONTROLLABLE SYNTHESIS; TIO2; LDH; UV; PHOTOACTIVITY; NANOPARTICLES; TEMPERATURE; NANOSHEETS; PRESSURE; FILMS;
D O I
10.1016/j.jtice.2018.07.031
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
In this work, a 3D-Ag/NiCo-LDHs photocatalyst was successfully prepared. Varies analytical techniques demonstrated that the Ag/NiCo-LDHs showed excellent photocatalytic activity than pure NiCo-LDHs, which may attribute the special structure of NiCo-LDHs with adsorption performance and surface plasma resonance effect (SPR) of Ag nanoparticles. Such flower-like structure of NiCo-LDHs, the petals staggered to form a plurality of independent reaction spaces to provide more reaction space and avoid the interaction between the reaction products. Meanwhile, combining the carbon quantum dots with the SPR of Ag nanoparticles can further enhance the photocatalytic activity. Based on the analysis, the possible photo catalytic mechanism was presented. (C) 2018 Taiwan Institute of Chemical Engineers. Published by Elsevier B.V. All rights reserved.
引用
收藏
页码:298 / 305
页数:8
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