Formation of silver nanoparticles in thin oxide layer on Si by negative-ion implantation

被引:19
作者
Arai, N
Tsuji, H [1 ]
Motono, M
Gotoh, Y
Adachi, K
Kotaki, H
Ishikawa, J
机构
[1] Kyoto Univ, Dept Elect Sci & Engn, Sakyo Ku, Kyoto 6068501, Japan
[2] Sharp Co Ltd, Adv Technol Res Lab, Tenri, Nara 6328567, Japan
关键词
metal nanoparticle; negative ion implantation; oxide film;
D O I
10.1016/S0168-583X(03)00801-2
中图分类号
TH7 [仪器、仪表];
学科分类号
0804 ; 080401 ; 081102 ;
摘要
Formation of nanoparticles in a 50-nm-thick SiO2 film on Si was conducted by silver negative ion implantation at 30 keV with various doses, and the state of nanoparticles in the thin oxide film was observed by a cross-sectional scanning TEM. The sample implanted with 1 x 10(15) ions/cm(2) showed nanoparticles with diameter of about 2-3 nn distributed in the middle of the SiO2 film on Si. The location of nanoparticles was in good agreement with the calculated profile by TRIM-DYN. Nanoparticles with various diameters of 4-8 nm formed in samples of 1 x 10(16) and 1 x 10(17) ions/cm(2). The size of silver nanoparticles was found to relate strongly to density of implanted atoms in the layer. (C) 2003 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:629 / 633
页数:5
相关论文
共 13 条
[2]   NEGATIVE-ION IMPLANTATION TECHNIQUE [J].
ISHIKAWA, J ;
TSUJI, H ;
TOYOTA, Y ;
GOTOH, Y ;
MATSUDA, K ;
TANJYO, M ;
SAKAI, S .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS, 1995, 96 (1-2) :7-12
[3]   Self-assembled two-dimensional distribution of nanoparticles with high-current Cu- implantation into insulators [J].
Kishimoto, N ;
Umeda, N ;
Takeda, Y ;
Lee, CG ;
Gritsyna, VT .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS, 1999, 148 (1-4) :1017-1022
[5]   Single electron charging of Sn nanocrystals in thin SiO2 film formed by low energy ion implantation [J].
Nakajima, A ;
Futatsugi, T ;
Horiguchi, N ;
Nakao, H ;
Yokoyama, N .
INTERNATIONAL ELECTRON DEVICES MEETING - 1997, TECHNICAL DIGEST, 1997, :159-162
[6]   MEASUREMENT OF NEGATIVE-ION-PRODUCTION EFFICIENCIES AND DEVELOPMENT OF A DC OPERATION SPUTTER-TYPE NEGATIVE-ION SOURCE [J].
TSUJI, H ;
ISHIKAWA, J .
REVIEW OF SCIENTIFIC INSTRUMENTS, 1992, 63 (04) :2488-2490
[7]   Contact angle lowering of polystyrene surface by silver-negative-ion implantation for improving biocompatibility and introduced atomic bond evaluation by XPS [J].
Tsuji, H ;
Satoh, H ;
Ikeda, S ;
Gotoh, Y ;
Ishikawa, J .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS, 1998, 141 (1-4) :197-201
[8]   Secondary electron emission and surface potential of SiO2 film surface by negative ion bombardment [J].
Tsuji, H ;
Gotoh, Y ;
Ishikawa, J .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS, 1998, 141 (1-4) :645-651
[9]   Fundamental study on powder-scattering in positive- and negative-ion implantation into powder materials [J].
Tsuji, H ;
Ishikawa, J ;
Itoh, H ;
Toyota, Y ;
Gotoh, Y .
APPLIED SURFACE SCIENCE, 1996, 100 :342-346
[10]   Negative-ion implanter for powders and its application to nanometer-sized metal particle formation in the surface of glass beads [J].
Tsuji, H ;
Kido, S ;
Sasaki, H ;
Gotoh, Y ;
Ishikawa, J .
REVIEW OF SCIENTIFIC INSTRUMENTS, 2000, 71 (02) :804-806