Electrochemical Transformation of CO2 to Value-Added Chemicals and Fuels

被引：47

作者：

Jia, Shunhan ^{[1
,2
]}

Ma, Xiaodong ^{[1
,2
]}

Sun, Xiaofu ^{[1
,2
]}

Han, Buxing ^{[1
,2
,3
]}

机构：

[1] Chinese Acad Sci, CAS Res Educ Ctr Excellence Mol Sci, Inst Chem, Beijing Natl Lab Mol Sci,CAS Key Lab Colloid & In, Beijing 100190, Peoples R China

[2] Univ Chinese Acad Sci, Sch Chem Sci, Beijing 100049, Peoples R China

[3] East China Normal Univ, Sch Chem & Mol Engn, Shanghai Key Lab Green Chem & Chem Proc, Shanghai 200062, Peoples R China

来源：

CCS CHEMISTRY | 2022年 / 4卷 / 10期

基金：

中国国家自然科学基金;

关键词：

carbon dioxide; green chemistry; green carbon science; electro-organic synthesis; catalysis; ELECTROCATALYTIC REDUCTION; CARBON-MONOXIDE; IONIC LIQUIDS; ASYMMETRIC ELECTROCARBOXYLATION; CYCLIC CARBONATES; EMERGING PLATFORM; ELECTROREDUCTION; ELECTROSYNTHESIS; DIOXIDE; CARBOXYLATION;

D O I：

10.31635/ccschem.022.202202094

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

CO2 is the main greenhouse gas and a renewable carbon resource. Electrochemical transformation of CO2 (CO2ET) to value-added chemicals and fuels is one of the promising routes to reduce CO2 emission and contributes to sustainability and carbon neutrality. In this review, we discuss recent developments on apparatuses used in CO2ET, electrocatalytic reactions of CO2 with water, organics, nitrogen, and nitrogen-containing compounds to synthesize chemicals and fuels by the construction of different chemical bonds (e.g., C-H, C-C, C-O, and C-N), and related reaction mechanisms. Also, an outlook was considered to highlight the opportunities and challenges in CO2ET.

引用

页码：3213 / 3229

页数：17

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