Synergistic photocatalytic dye mitigation and bacterial disinfection using carbon quantum dots decorated dual Z-scheme Manganese Indium Sulfide/Cuprous Oxide/Silver oxide heterojunction

被引:111
作者
Sharma, Sheetal [1 ]
Dutta, Vishal [1 ]
Raizada, Pankaj [1 ]
Thakur, Vijay Kumar [2 ,9 ]
Saini, Adesh K. [3 ]
Mittal, Divya [3 ]
Van-Huy Nguyen [4 ]
Ahamad, Tansir [5 ]
Chinh Chien Nguyen [6 ,7 ]
Kim, Soo Young [8 ]
Quyet Van Le [8 ]
Singh, Pardeep [1 ]
机构
[1] Shoolini Univ, Sch Adv Chem Sci, Solan 173212, Himachal Prades, India
[2] Scotlands Rural Coll SRUC, Biorefining & Adv Mat Res Ctr, Edinburgh, Midlothian, Scotland
[3] Maharishi Markandeshwar Deemed Univ, Dept Biotechnol MMEC & Cent Res Cell, Ambala 133207, HR, India
[4] Binh Duong Univ, Fac Biotechnol, Thu Dau Mot, Vietnam
[5] King Saud Univ, Coll Sci, Dept Chem, Riyadh, Saudi Arabia
[6] Duy Tan Univ, Inst Res & Dev, Da Nang 550000, Vietnam
[7] Duy Tan Univ, Fac Environm Chem Engn, Da Nang 550000, Vietnam
[8] Korea Univ, Fac Dept Mat Sci & Engn, 145 Anam Ro, Seoul 02841, South Korea
[9] Univ Petr & Energy Studies UPES, Sch Engn, Dehra Dun 248007, Uttarakhand, India
基金
新加坡国家研究基金会;
关键词
Dual Z-scheme; Tandem charge transfer; MO removal; E. coli disinfection;
D O I
10.1016/j.matlet.2022.131716
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
A novel CQDs decorated MnIn2S4/Cu2O/Ag2O dual Z-scheme tandem hybrid is fabricated via hydrothermal method for MO removal and E. coli disinfection under visible light illumination. CQDs shuttle electrons in CQDsMnIn(2)S(4)/Cu2O/Ag2O interface via dual Z-scheme electron transferal route which lead to upgrade in charge separation and visible light absorption. The Z-scheme hybrid displayed best catalytic inactivation performance of E. coli and degradation of MO which totally disinfect bacteria within 3 h and displayed 98.6% of MO degradation in 70 min in visible light radiation. The unique dual Z-scheme junction supports enhanced redox capabilities, prolong lifespan of photo-excitons, stability, spatial separation and enhanced visible light absorption.
引用
收藏
页数:5
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