The activation of heterogeneous Fenton-type catalyst Fe-MFI

被引：37
|
作者：
Parkhomchuk, E. V. [1 ]
Vanina, M. P. [1 ]
Preis, S. [2 ]
机构：
[1] Boreskov Inst Catalysis, Novosibirsk 630090, Russia
[2] Lappeenranta Univ Technol, Lappeenranta 53850, Finland
来源：
CATALYSIS COMMUNICATIONS | 2008年 / 9卷 / 03期
基金：
芬兰科学院;
关键词：
hydrogen peroxide; Fenton; heterogeneous catalysis; MFI; zeolite activation;
D O I：
10.1016/j.catcom.2007.07.009
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
The activation of iron-containing zeolite of MFI structure with mineral and carboxylic acids in heterogeneous Fenton reaction was experimentally studied. The catalytic activity of the zeolite was tested in the hydrogen peroxide decomposition reaction. The activation effect of acids was observed in the following decreasing order: oxalic > acetic > hydrochloric > formic. The catalyst pre-treatment with nitric acid was ineffective. Optimum conditions for the most effective pre-treatment of the zeolite with aqueous oxalic acid solutions were established. (c) 2007 Elsevier B.V. All rights reserved.
引用
收藏
页码：381 / 385
页数：5
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