Capture of CO2 from coal-fired power plant with NaOH solution in a continuous

被引:10
作者
Chen, Pao Chi [1 ]
Huang, C. F. [2 ]
Chen, Hsiao-Wei [3 ]
Yang, Ming-Wei [3 ]
Tsao, Chih-Ming [3 ]
机构
[1] Lunghwa Univ Sci Technol, Dept Chem & Mat Engn, Taoyuan, Taiwan
[2] Lunghwa Univ Sci Technol, Taoyuan, Taiwan
[3] Taiwan Power Conpany, Taoyuan, Taiwan
来源
INTERNATIONAL CONFERENCE ON APPLIED ENERGY, ICAE2014 | 2014年 / 61卷
关键词
Taguchi Method; overall mass-transfer coefficient; two-film model; carbon capture; ABSORPTION;
D O I
10.1016/j.egypro.2014.12.186
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A continuous pilot-scale bubble-column scrubber with NaOH as the absorbent was used to explore the capture of CO2 gas from a coal-fired power plant. The experimental design was based on the results of previous study. The diameter of the column was 20 cm and the height of the column was 2.4 m. According to the S/N ratio, parameters, including absorption rate (R-A), absorption efficiency (E), overall mass-transfer coefficient (K(G)a) and ratio of the gas-liquid flow rate (R), were selected for Taguchi analysis to obtain optimum conditions. A total of eleven experiments were carried out to verify the optimum conditions here. The range of the gas-flow rate (Q(g)) and liquid-flow rate (Q(LT)) conducted in this work were 48-192 L/min and 1.6-10 L/min, respectively. The input gas concentrations were 9-12.2%. Using a steady-state material balance with a two-film model, R-A and K(G)a could be determined. The results showed that E, R-A and K(G)a were in the range of 30-98%, 1.03x10-(4).11.48x10(-4) molls-L and 0.018-0.058 1/s, respectively. The obtained scrubbing factors (phi) were 0.00285-0.146 mol/mol-L, while R was in the range of 0.23-24.14. The dynamic behavior of the scrubber was also discussed in this study. The results could be used as a basis for commercial scale operation for the carbon capture at a power plant as well as microalgae cultivation.
引用
收藏
页码:1660 / 1664
页数:5
相关论文
共 9 条
[1]   Comprehensive study of the kinetics of the oxidative degradation of CO2 loaded and concentrated aqueous monoethanolamine (MEA) with and without sodium metavanadate during CO2 absorption from flue gases [J].
Bello, A ;
Idem, RO .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2006, 45 (08) :2569-2579
[2]  
Chen P.-C., 2012, Absorption of Carbon Dioxide in a Bubble-Column Scrubber, Greenhouse Gases - Capturing
[3]  
Chen Pao Chi, 2013, ABSORPTION CO2 USING
[4]   Scrubbing of CO2 greenhouse gases, accompanied by precipitation in a continuous bubble-column scrubber [J].
Chen, Pao-Chi ;
Shi, Welly ;
Du, Ruby ;
Chen, Vanessa .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2008, 47 (16) :6336-6343
[5]   Experimental study on capturing CO2 greenhouse gas by ammonia scrubbing [J].
Diao, YF ;
Zheng, XY ;
He, BS ;
Chen, CH ;
Xu, XC .
ENERGY CONVERSION AND MANAGEMENT, 2004, 45 (13-14) :2283-2296
[6]   Microalgae: The Potential for Carbon Capture [J].
Sayre, Richard .
BIOSCIENCE, 2010, 60 (09) :722-727
[7]   Progress in carbon dioxide separation and capture: A review [J].
Yang, Hongqun ;
Xu, Zhenghe ;
Fan, Maohong ;
Gupta, Rajender ;
Slimane, Rachid B. ;
Bland, Alan E. ;
Wright, Ian .
JOURNAL OF ENVIRONMENTAL SCIENCES, 2008, 20 (01) :14-27
[8]   Semi-batch absorption and regeneration studies for CO2 capture by aqueous ammonia [J].
Yeh, JT ;
Resnik, KP ;
Rygle, K ;
Pennline, HW .
FUEL PROCESSING TECHNOLOGY, 2005, 86 (14-15) :1533-1546
[9]   Carbon dioxide capture capacity of sodium hydroxide aqueous solution [J].
Yoo, Miran ;
Han, Sang-Jun ;
Wee, Jung-Ho .
JOURNAL OF ENVIRONMENTAL MANAGEMENT, 2013, 114 :512-519