Quantile regression of indoor air concentrations of volatile organic compounds (VOC)

被引:67
作者
Schlink, Uwe [1 ]
Thiem, Alexander [1 ]
Kohajda, Tibor [1 ]
Richter, Matthias [1 ]
Strebel, Kathrin [1 ]
机构
[1] UFZ Helmholtz Ctr Environm Res, D-04318 Leipzig, Germany
关键词
Volatile organic compounds; Indoor air quality; Quantile regression; Modifying factors; SUBURBAN NEIGHBORHOODS; PERSONAL EXPOSURES; SEASONAL CYCLE; URBAN; HYDROCARBONS; INDUSTRIAL;
D O I
10.1016/j.scitotenv.2009.12.002
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
There are many factors determining the concentration of volatile organic compounds (VOCs) in indoor air. On the basis of 601 population-based measurements we develop an explicit exposure model that includes factors, such as renovation, furniture, flat size, smoking, and education level of the occupants. As a novel method for the evaluation of concentrations of indoor air pollutants we use quantile regression, which has the advantages of robustness against non-Gaussian distributions (and outliers) and can adjust for unbalanced frequencies of observations. The applied bi- and multivariate quantile regressions provide (1) the VOC burden that is representative for the population of Leipzig, Germany. and (2) an inter-comparison of the effects of the studied factors and their levels. As a result, we find strong evidence for factors of general impact on most VOC components, such as the season, flooring, the type of the room, and the size of the apartment. Other impact factors are very specific to the VOC components. For example, wooden flooring (parquet) and new furniture increase the concentration of terpenes as well as the modifying factors high education and sampling in the child's room. Smokers ventilate their flats in an extent that in general reduces the VOC concentrations, except for benzene (contained in tobacco smoke), which is still higher in smoking than in non-smoking flats. Very often dampness is associated with an increased VOC burden in indoor air. An investigation of mixtures emphasises a high burden of co-occurring terpenes in very small and very large apartments. (C) 2009 Elsevier B.V. All rights reserved.
引用
收藏
页码:3840 / 3851
页数:12
相关论文
共 38 条
[1]  
BAUMANN R, 2003, BEWERTUNG INNENRAUML
[2]   PASSIVE SAMPLING FOR VOLATILE ORGANIC-COMPOUNDS (VOCS) IN AIR AT ENVIRONMENTALLY RELEVANT CONCENTRATION LEVELS [J].
BEGEROW, J ;
JERMANN, E ;
KELES, T ;
RANFT, U ;
DUNEMANN, L .
FRESENIUS JOURNAL OF ANALYTICAL CHEMISTRY, 1995, 351 (06) :549-554
[3]   CONCENTRATIONS OF VOLATILE ORGANIC-COMPOUNDS IN INDOOR AIR - A REVIEW [J].
BROWN, SK ;
SIM, MR ;
ABRAMSON, MJ ;
GRAY, CN .
INDOOR AIR-INTERNATIONAL JOURNAL OF INDOOR AIR QUALITY AND CLIMATE, 1994, 4 (02) :123-134
[4]   HUMAN ACTIVITIES AS SOURCES OF VOLATILE ORGANIC-COMPOUNDS IN RESIDENTIAL ENVIRONMENTS [J].
CLOBES, AL ;
ANANTH, GP ;
HOOD, AL ;
SCHROEDER, JA ;
LEE, KA .
ANNALS OF THE NEW YORK ACADEMY OF SCIENCES-SERIES, 1992, 641 :79-86
[5]   Ethnicity, housing and personal factors as determinants of VOC exposures [J].
D'Souza, Jennifer C. ;
Jia, Chunrong ;
Mukherjee, Bhrarmar ;
Batterman, Stuart .
ATMOSPHERIC ENVIRONMENT, 2009, 43 (18) :2884-2892
[6]   Measured and modeled personal exposures to and risks from volatile organic compounds [J].
Dodson, Robin E. ;
Houseman, E. Andres ;
Levy, Jonathan I. ;
Spengler, John D. ;
Shine, James P. ;
Bennett, Deborah H. .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2007, 41 (24) :8498-8505
[7]   Benzene exposure in Helsinki, Finland [J].
Edwards, RD ;
Jantunen, MJ .
ATMOSPHERIC ENVIRONMENT, 2001, 35 (08) :1411-1420
[8]   VOLATILE HALOGENATED HYDROCARBONS IN URBAN ATMOSPHERE AND IN HUMAN BLOOD [J].
GILLI, G ;
BONO, R ;
SCURSATONE, E .
ARCHIVES OF ENVIRONMENTAL HEALTH, 1990, 45 (02) :101-106
[9]   Spatiotemporal distribution of airborne mould spores in apartments [J].
Herbarth, O ;
Schlink, U ;
Müller, A ;
Richter, M .
MYCOLOGICAL RESEARCH, 2003, 107 :1361-1371
[10]   Background concentrations of individual and total volatile organic compounds in residential indoor air of Schleswig-Holstein, Germany [J].
Hippelein, M .
JOURNAL OF ENVIRONMENTAL MONITORING, 2004, 6 (09) :745-752