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Spatial charge separation on strongly coupled 2D-hybrid of rGO/La2Ti2O7/NiFe-LDH heterostructures for highly efficient noble metal free photocatalytic hydrogen generation
被引:122
作者:

Boppella, Ramireddy
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Ewha Womans Univ, Dept Chem & Nano Sci, 52 Ewhayeodae Gil, Seoul 03760, South Korea
Yonsei Univ, Dept Mat Sci & Engn, 50 Yonsei Ro, Seoul 03722, South Korea Ewha Womans Univ, Dept Chem & Nano Sci, 52 Ewhayeodae Gil, Seoul 03760, South Korea

Choi, Chi Hun
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Ewha Womans Univ, Dept Chem & Nano Sci, 52 Ewhayeodae Gil, Seoul 03760, South Korea Ewha Womans Univ, Dept Chem & Nano Sci, 52 Ewhayeodae Gil, Seoul 03760, South Korea

Moon, Jooho
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Yonsei Univ, Dept Mat Sci & Engn, 50 Yonsei Ro, Seoul 03722, South Korea Ewha Womans Univ, Dept Chem & Nano Sci, 52 Ewhayeodae Gil, Seoul 03760, South Korea

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机构:
[1] Ewha Womans Univ, Dept Chem & Nano Sci, 52 Ewhayeodae Gil, Seoul 03760, South Korea
[2] Yonsei Univ, Dept Mat Sci & Engn, 50 Yonsei Ro, Seoul 03722, South Korea
基金:
新加坡国家研究基金会;
关键词:
Lanthanum titanate;
NiFe-LDH;
Reduced graphene oxide;
Semiconductor photocatalyst;
Dual co-catalysts;
Water splitting;
LAYERED DOUBLE HYDROXIDES;
NANOWIRE ARRAYS;
COMPOSITE PHOTOCATALYST;
H-2-PRODUCTION ACTIVITY;
ENHANCED PHOTOACTIVITY;
WATER;
GRAPHENE;
SEMICONDUCTOR;
COCATALYSTS;
EVOLUTION;
D O I:
10.1016/j.apcatb.2018.07.063
中图分类号:
O64 [物理化学(理论化学)、化学物理学];
学科分类号:
070304 ;
081704 ;
摘要:
Developing photocatalysts with effective charge separation and fast surface reaction kinetics is crucial to realizing efficient photocatalytic water splitting. In this study, we report a strongly coupled two-dimensionalternary-heterostructured photocatalyst by sequentially introducing reduced graphene oxide (rGO) and NiFe-layered double hydroxide (NiFe-LDH) on the surface of lanthanum titanate (LTO) via a facile hydrothermal and electrostatic self-assembly methodology, respectively. The synthesized 2D-rGO/LTO/NiFe-LDH photocatalyst showed remarkable photocatalytic H-2 evolution activity under simulated light irradiation, even without expensive Pt cocatalyst. The enhancement of photocatalytic activity could be attributed to the efficient interfacial charge transfer at the rGO/LTO heterojunction interface, and the enhanced hole (h(+)) trapping ability of NiFe-LDH cocatalyst at the LTO/NiFe-LDH interface, respectively. These attributes could effectively enlarge the life time of photo-generated electron-hole pairs, and increase the electron density for hydrogen production. The optimal rGO/LTO/NiFe-LDH nanocomposite remain sustained even after four successive experimental runs, without apparent change in the H-2 evolution rate. The present work elucidates a new strategy to maximize the efficiency via synergetic effect of incorporating rGO and NiFe-LDH as dual cocatalysts, and shows a feasible strategy of using earth-abundant materials as cocatalysts to enhance the overall photocatalytic water splitting reactions.
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页码:178 / 186
页数:9
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