Atomic carbon chains as spin-transmitters: An ab initio transport study

被引:26
作者
Furst, J. A. [1 ]
Brandbyge, M. [1 ]
Jauho, A. -P. [1 ,2 ]
机构
[1] Tech Univ Denmark, NanoDTU, Dept Micro & Nanotechnol, DTU Nanotech, DK-2800 Lyngby, Denmark
[2] Aalto Univ, Dept Appl Phys, FI-00076 Aalto, Finland
关键词
GRAPHENE; NANOTUBE; STATE;
D O I
10.1209/0295-5075/91/37002
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
An atomic carbon chain joining two graphene flakes was recently realized in a ground-breaking experiment by Jin et al. (Phys. Rev. Lett., 102 (2009) 205501). We present ab initio results for the electron transport properties of such chains and demonstrate complete spin-polarization of the transmission in large energy ranges. The effect is due to the spin-polarized zig-zag edge terminating each graphene flake causing a spin-splitting of the graphene pi(z) bands, and the chain states. Transmission occurs when the graphene p-states resonate with similar states in the strongly hybridized edges and chain. This effect should in general hold for any p-conjugated molecules bridging the zig-zag edges of graphene electrodes. The polarization of the transmission can be controlled by chemically or mechanically modifying the molecule, or by applying an electrical gate. Copyright (c) EPLA, 2010
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页数:5
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