Batch versus continuous feeding strategies for pharmaceutical removal by subsurface flow constructed wetland

被引：78

作者：

Zhang, Dong Qing ^{[1
]}

Gersberg, Richard M. ^{[2
]}

Zhu, Junfei ^{[1
]}

Hua, Tao ^{[1
]}

Jinadasa, K. B. S. N. ^{[3
]}

Tan, Soon Keat ^{[4
]}

机构：

[1] Nanyang Technol Univ, DHI NTU Ctr, Nanyang Environm & Water Res Inst, Singapore 639798, Singapore

[2] San Diego State Univ, Grad Sch Publ Hlth, San Diego, CA 92182 USA

[3] Univ Peradeniya, Dept Civil Engn, Peradeniya 20400, Sri Lanka

[4] Nanyang Technol Univ, Maritime Res Ctr, Sch Civil & Environm Engn, Singapore 639798, Singapore

来源：

ENVIRONMENTAL POLLUTION | 2012年 / 167卷

关键词：

Batch (drain and fill); Continuous flow; Pharmaceutical; First-order kinetics; Log D-ow; PERSONAL CARE PRODUCTS; WASTE-WATER TREATMENT; CLOFIBRIC ACID; PERFORMANCE; IBUPROFEN; PLANT; FATE; CARBAMAZEPINE; DEGRADATION; METABOLITES;

D O I：

10.1016/j.envpol.2012.04.004

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

This study evaluated the effect of continuous and batch feeding on the removal of 8 pharmaceuticals (carbamazepine, naproxen, diclofenac, ibuprofen, caffeine, salicylic acid, ketoprofen and clofibric acid) from synthetic wastewater in mesocosm-scale constructed wetlands (CWs). Both loading modes were operated at hydraulic application rates of 5.6 cm day(-1) and 2.8 cm day(-1). Except for carbamazepine, clofibric acid and naproxen, removal in CWs was significantly (p < 0.05) enhanced under the batch versus continuous mode. For all compounds tested except naproxen, values for first-order decay constants (k) for drain and fill operation were higher than that for the continuous mode of operation. Correlation between the distribution coefficient (log D-ow) and removal efficiencies of pharmaceutical compounds in the CWs, showed that pharmaceutical removal efficiency was significantly (p < 0.1) and inversely correlated with log D-ow value, but not with log K-ow value. (C) 2012 Elsevier Ltd. All rights reserved.

引用

页码：124 / 131

页数：8

共 53 条

[11]

ChemAxon, 2007, MARV CALC PLUG DEM

[12]

Clesceri L.S., 1989, STANDARD METHODS EXA, V17th

[13] Pharmaceuticals and personal care products in the environment: Agents of subtle change? [J].

Daughton, CG ;

Ternes, TA .

ENVIRONMENTAL HEALTH PERSPECTIVES, 1999, 107 :907-938

[14] Preliminary media screening for application in the removal of clofibric acid, carbamazepine and ibuprofen by SSF-constructed wetlands [J].

Dordio, Ana V. ;

Candeias, A. J. Estevao ;

Pinto, A. P. ;

da Costa, C. Teixeira ;

Carvalho, A. J. Palace .

ECOLOGICAL ENGINEERING, 2009, 35 (02) :290-302

[15]

Fent K, 2006, AQUAT TOXICOL, V76, P122, DOI 10.1016/j.aquatox.2005.09.009

[16] Pilot survey monitoring pharmaceuticals and related compounds in a sewage treatment plant located on the Mediterranean coast [J].

Gomez, M. J. ;

Bueno, M. J. Martinez ;

Lacorte, S. ;

Fernandez-Alba, A. R. ;

Aguera, A. .

CHEMOSPHERE, 2007, 66 (06) :993-1002

[17] Occurrence, fate, and removal of pharmaceutical residues in the aquatic environment: a review of recent research data [J].

Heberer, T .

TOXICOLOGY LETTERS, 2002, 131 (1-2) :5-17

[18] Assessment of full-scale natural systems for the removal of PPCPs from wastewater in small communities [J].

Hijosa-Valsero, Maria ;

Matamoros, Victor ;

Martin-Villacorta, Javier ;

Becares, Eloy ;

Bayona, Josep M. .

WATER RESEARCH, 2010, 44 (05) :1429-1439

[19] Occurrence of psychoactive stimulatory drugs in wastewaters in north-eastern Spain [J].

Huerta-Fontela, Maria ;

Galceran, Maria Teresa ;

Martin-Alonso, Jordi ;

Ventura, Francesc .

SCIENCE OF THE TOTAL ENVIRONMENT, 2008, 397 (1-3) :31-40

[20]

IWA Specialist Group on Use of Macrophytes inWater Pollution, 2000, 8 IWA SPEC GROUP US

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