Fabrication of a Microcavity Prepared by Remote Epitaxy over Monolayer Molybdenum Disulfide

被引:20
作者
Kim, Yeonhoo [1 ,2 ]
Watt, John [1 ]
Ma, Xuedan [3 ]
Ahmed, Towfiq [4 ]
Kim, Suhyun [5 ]
Kang, Kibum [5 ]
Luk, Ting S. [6 ]
Hong, Young Joon [7 ]
Yoo, Jinkyoung [1 ]
机构
[1] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA
[2] Korea Res Inst Stand & Sci KRISS, Interdisciplinary Mat Measurement Inst, Daejeon 34133, South Korea
[3] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA
[4] Los Alamos Natl Lab, T-4, Los Alamos, NM 87545 USA
[5] Korea Adv Inst Sci & Technol KAIST, Dept Mat Sci & Engn, Daejeon 34141, South Korea
[6] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA
[7] Sejong Univ, Dept Nanotechnol & Adv Mat Engn, Seoul 05006, South Korea
关键词
remote epitaxy; microcavity; two-dimensional material; transition metal dichalcogenides; polarity inversion; whispering-gallery-mode; TOTAL-ENERGY CALCULATIONS; CHARGE-TRANSFER; WAFER-SCALE; GRAPHENE; MOS2; HETEROSTRUCTURES; INTEGRATION; INVERSION;
D O I
10.1021/acsnano.1c08779
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Advances in epitaxy have enabled the preparation of high-quality material architectures consisting of incommensurate components. Remote epitaxy based on lattice transparency of atomically thin graphene has been intensively studied for cost-effective advanced device manufacturing and heterostructure formation. However, remote epitaxy on non-graphene two-dimensional (2D) materials has rarely been studied even though it has a broad and immediate impact on various disciplines, such as many-body physics and the design of advanced devices. Herein, we report remote epitaxy of ZnO on monolayer MoS2 and the realization of a whispering-gallery-mode (WGM) cavity composed of a single crystalline ZnO nanorod and monolayer MoS2. Cross-sectional transmission electron microscopy and first-principles calculations revealed that the nongraphene 2D material interacted with overgrown and substrate layers and also exhibited lattice transparency. The WGM cavity embedding monolayer MoS2 showed enhanced luminescence of MoS2 and multimodal emission.
引用
收藏
页码:2399 / 2406
页数:8
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