Short-lived fission product measurements from >0.1 MeV neutron-induced fission using boron carbide

被引:8
作者
Finn, Erin [1 ]
Metz, Lori [1 ]
Greenwood, Larry [1 ]
Pierson, Bruce [1 ,2 ]
Friese, Judah [1 ]
Kephart, Rosara [1 ]
Kephart, Jeremy [1 ]
机构
[1] Pacific NW Natl Lab, Richland, WA 99352 USA
[2] Univ Michigan, Ann Arbor, MI 48109 USA
关键词
Boron carbide; Short-lived fission products; Gamma spectra; Fast fission energy neutrons; GAMMA-RAYS; YIELDS;
D O I
10.1007/s10967-012-1652-y
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
A boron carbide shield was designed, custom fabricated, and used to create a fast fission energy neutron spectrum. The fissionable isotopes U-233,U- 235,U- 238, Np-237, and Pu-239 were separately placed inside of this shield and irradiated under pulsed conditions at the Washington State University 1 MW TRIGA reactor. A unique set of fission product gamma spectra were collected at short times (4 min to 1 week) post-fission. Gamma spectra were collected on single-crystal high purity germanium detectors and on Pacific Northwest National Laboratory's Direct Simultaneous Measurement system composed of HPGe detectors connected in coincidence. This work defines the experimental methods used to produce and collect the gamma data, and demonstrates the validity of the measurements. It is important to fully document this information so the data can be used with high confidence for the advancement of nuclear science and non-proliferation applications. The gamma spectra collected in these and other experiments are publicly available at https://spcollab.pnnl.gov/sites/gammadata/default.aspx or via the link at http://rdnsgroup.pnnl.gov. A revised version of this publication will be posted with the data to make the experimental details available to those using the data.
引用
收藏
页码:267 / 272
页数:6
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