MoS2/Ti3C2 heterostructure for efficient visible-light photocatalytic hydrogen generation

被引：79

作者：

Zhang, Juhui ^{[1
]}

Xing, Chao ^{[1
]}

Shi, Feng ^{[1
]}

机构：

[1] Shandong Univ Sci & Technol, Sch Mat Sci & Engn, Qingdao 266590, Peoples R China

来源：

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY | 2020年 / 45卷 / 11期

基金：

中国国家自然科学基金;

关键词：

Photocatalytic hydrogen evolution; MoS2; spheres; Ti3C2; MXene; Heterostructure; Photogenerated electrons; Hydrothermal methods; TRANSITION-METAL CARBIDES; MOS2; NANOSHEETS; EVOLUTION; WATER; CAPACITANCE;

D O I：

10.1016/j.ijhydene.2019.12.109

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

The MoS2/Ti3C2 catalyst with a unique sphere/sheet structure were prepared by hydro thermal method. The MoS2/Ti3C2 heterostructure loading 30% Ti3C2 has a maximum hydrogen production rate of 6144.7 mu mol g(-1) h(-1), which are 2.3 times higher than those of the pure MoS2. The heterostructure maintains a high catalytic activity within 4 cycles. The heterostructure not only effectively reduce the recombination of photogenerated electrons and holes, but also provide more activation sites, which promotes the photocatalytic hydrogen evolution reaction (HER). These works can provide reference for the development of efficient catalysts in photocatalytic hydrogen evolution. (C) 2019 Published by Elsevier Ltd on behalf of Hydrogen Energy Publications LLC.

引用

页码：6291 / 6301

页数：11

共 50 条

[31] Highly efficient visible-light photocatalytic activity of MoS2-TiO2 mixtures hybrid photocatalyst and functional properties [J].

Sabarinathan, M. ;

Harish, S. ;

Archana, J. ;

Navaneethan, M. ;

Ikeda, H. ;

Hayakawa, Y. .

RSC ADVANCES, 2017, 7 (40) :24754-24763

[32] Noble-metal-free MoS2/Ta3N5 heterostructure photocatalyst for hydrogen generation [J].

Xiao, Mu ;

Luo, Bin ;

Thaweesak, Supphasin ;

Wang, Lianzhou .

PROGRESS IN NATURAL SCIENCE-MATERIALS INTERNATIONAL, 2018, 28 (02) :189-193

[33] Efficient visible-light photocatalytic ozonation for dye degradation using Fe2O3/MoS2 nanocomposite [J].

Bagheri, Fatemeh ;

Chaibakhsh, Naz .

SEPARATION SCIENCE AND TECHNOLOGY, 2021, 56 (17) :3022-3032

[34] High-performance MoS2/CdS nanodiamonds for photocatalytic hydrogen evolution under visible light irradiation [J].

Fu, Haitao ;

Zhao, Hongming ;

Yang, Xiaohong ;

Xiong, Shixian ;

An, Xizhong .

POWDER TECHNOLOGY, 2022, 406

[35] Synthesis of Ag/hybridized 1T-2H MoS2/TiO2 heterostructure for enhanced visible-light photocatalytic activity [J].

Alido, John Peter M. ;

Sari, Fitri Nur Indah ;

Ting, Jyh-Ming .

CERAMICS INTERNATIONAL, 2019, 45 (17) :23651-23657

[36] Morphology-controlled synthesis of TiO2/MoS2 nanocomposites with enhanced visible-light photocatalytic activity [J].

Sun, Yuanqing ;

Lin, Huihui ;

Wang, Chuanxi ;

Wu, Qian ;

Wang, Xiaojie ;

Yang, Minghui .

INORGANIC CHEMISTRY FRONTIERS, 2018, 5 (01) :145-152

[37] OD/2D nanocomposite visible light photocatalyst for highly stable and efficient hydrogen generation via recrystallization of CdS on MoS2 nanosheets [J].

Ma, Fukun ;

Wu, Yongzhong ;

Shao, Yongliang ;

Zhong, Yueyao ;

Lv, Jiaxin ;

Hao, Xiaopeng .

NANO ENERGY, 2016, 27 :466-474

[38] In situ fabrication of 2D/3D g-C3N4/Ti3C2 (MXene) heterojunction for efficient visible-light photocatalytic hydrogen evolution [J].

Li, Jinmao ;

Zhao, Li ;

Wang, Shimin ;

Li, Jin ;

Wang, Guohong ;

Wang, Juan .

APPLIED SURFACE SCIENCE, 2020, 515

[39] Layered BiOBr/Ti3C2 MXene composite with improved visible-light photocatalytic activity [J].

Liu, Chao ;

Xu, Qixiang ;

Zhang, Qinfang ;

Zhu, Yisong ;

Ji, Mingwei ;

Tong, Zhiwei ;

Hou, Wenhua ;

Zhang, Yu ;

Xu, Jianguang .

JOURNAL OF MATERIALS SCIENCE, 2019, 54 (03) :2458-2471

[40] Interfacial Charge Transfer Effects of MoS2/α-Fe2O3 Nano-Heterojunction and Efficient Photocatalytic Hydrogen Evolution under Visible-Light Irradiation [J].

Tien, Tsung-Mo ;

Chen, Edward L. .

NANOMATERIALS, 2023, 13 (20)

← 1 2 3 4 5 →