MoS2 nanosheets encapsulating TiO2 hollow spheres with enhanced photocatalytic activity for nitrophenol reduction

被引:24
作者
Guo, Na [1 ,2 ]
Zeng, Ying [1 ,2 ]
Li, Haiyan [1 ]
Xu, Xingjian [1 ]
Yu, Hongwen [1 ]
机构
[1] Chinese Acad Sci, Northeast Inst Geog & Agroecol, 4888 Shengbei Rd, Changchun 130102, Jilin, Peoples R China
[2] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
关键词
MoS2; TiO2; Composite materials; Interfaces; 4-Aminophenol; REDUCED GRAPHENE OXIDE; 4-NITROPHENOL; DEGRADATION; COMPOSITES; NANOPARTICLES; NANOCRYSTALS; GENERATION;
D O I
10.1016/j.matlet.2017.08.068
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Crumpled MoS2 nanosheet encapsulating TiO2 hollow spheres (HT@M-0.8) core@shell three-dimensional (3D) heterojunction are synthesized successfully by in situ growth MoS2 on the surface of TiO2 through hydrothermal process. The core with a hollow structure enhanced light adsorption by multiple reflections in the available inner void space. The outer crumpled MoS2 can increase surface area of the composite. The photocatalytic reduction of HT@M-0.8 towards 4-nitrophenol is 99.35%, which is much higher than that of pure TiO2 and MoS2. The enhanced photocatalytic activity of HT@M-0.8 attributes to relative low recombination rate of the photogenerated electron-hole pairs. (C) 2017 Elsevier B.V. All rights reserved.
引用
收藏
页码:417 / 420
页数:4
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