Microphysical properties of Antarctic polar stratospheric clouds and their dependence on tropospheric cloud systems

被引:18
作者
Adhikari, Loknath [1 ]
Wang, Zhien [1 ]
Liu, Dong [1 ,2 ]
机构
[1] Univ Wyoming, Dept Atmospher Sci, Laramie, WY 82071 USA
[2] Chinese Acad Sci, Key Lab Atmospher Composit & Opt Radiat, Hefei, Peoples R China
关键词
NITRIC-ACID TRIHYDRATE; LIDAR OBSERVATIONS; ARCTIC STRATOSPHERE; SULFATE AEROSOLS; OZONE DEPLETION; PARTICLES; WINTER; NAT; DENITRIFICATION; CLIMATOLOGY;
D O I
10.1029/2009JD012125
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) and CloudSat satellite measurements are used to investigate the impact of tropospheric high and deep clouds on the microphysical properties of polar stratospheric clouds (PSCs) over Antarctica during the 2006 and 2007 winters. Based on the attenuated lidar scattering ratio and PSC depolarization ratio (delta'), PSCs are classified into supercooled ternary solution (STS), Mix 1, Mix 2, and ice classes with significantly different microphysical properties in terms of the PSC backscattering coefficient (beta(532)) for 532 nm, the color ratio (beta(1064)/beta(532)), and delta'. In the early stages of the PSC season, STS accounts for more than 50% of the total PSCs, but the Mix 1, Mix 2, and ice classes become more common in the late season. During the late PSC season, close to 70% of PSCs are formed in association with high and deep tropospheric cloud systems, indicating the important role of tropospheric weather systems in Antarctic PSC formation. Tropospheric cloud systems also affect the microphysical properties of PSCs by affecting the relative occurrence of different PSC classes, especially during September and October. Our results also show that there are noticeable differences in color ratio and beta(532) (at the 0.05 significance level) for the ice class and Mix 2 (late season only) for PSCs associated and not associated with high and deep tropospheric cloud systems. These results indicate that the impact of tropospheric meteorology on PSC formation should be fully considered to better understand interannual variations and recovery of the Antarctic ozone hole.
引用
收藏
页数:11
相关论文
共 45 条
[11]   Sensitivity of Arctic ozone loss to polar stratospheric cloud volume and chlorine and bromine loading in a chemistry and transport model [J].
Douglass, A. R. ;
Stolarski, R. S. ;
Strahan, S. E. ;
Polansky, B. C. .
GEOPHYSICAL RESEARCH LETTERS, 2006, 33 (17)
[12]   ANALYSIS OF THE PHYSICAL STATE OF ONE ARCTIC POLAR STRATOSPHERIC CLOUD BASED ON OBSERVATIONS [J].
DRDLA, K ;
TABAZADEH, A ;
TURCO, RP ;
JACOBSON, MZ ;
DYE, JE ;
TWOHY, C ;
BAUMGARDNER, D .
GEOPHYSICAL RESEARCH LETTERS, 1994, 21 (23) :2475-2478
[13]   The detection of large HNO3-containing particles in the winter arctic stratosphere [J].
Fahey, DW ;
Gao, RS ;
Carslaw, KS ;
Kettleborough, J ;
Popp, PJ ;
Northway, MJ ;
Holecek, JC ;
Ciciora, SC ;
McLaughlin, RJ ;
Thompson, TL ;
Winkler, RH ;
Baumgardner, DG ;
Gandrud, B ;
Wennberg, PO ;
Dhaniyala, S ;
McKinney, K ;
Peter, T ;
Salawitch, RJ ;
Bui, TP ;
Elkins, JW ;
Webster, CR ;
Atlas, EL ;
Jost, H ;
Wilson, JC ;
Herman, RL ;
Kleinböhl, A ;
von König, M .
SCIENCE, 2001, 291 (5506) :1026-1031
[14]   A unified, long-term, high-latitude stratospheric aerosol and cloud database using SAM II, SAGE II, and POAM II/III data: Algorithm description, database definition, and climatology [J].
Fromm, M ;
Alfred, J ;
Pitts, M .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D12)
[15]   Observations of Antarctic polar stratospheric clouds by POAM II: 1994-1996 [J].
Fromm, MD ;
Lumpe, JD ;
Bevilacqua, RM ;
Shettle, EP ;
Hornstein, J ;
Massie, ST ;
Fricke, KH .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1997, 102 (D19) :23659-23672
[16]   An analysis of Polar Ozone and Aerosol Measurement (POAM) II Arctic polar stratospheric cloud observations, 1993-1996 [J].
Fromm, MD ;
Bevilacqua, RM ;
Hornstein, J ;
Shettle, E ;
Hoppel, K ;
Lumpe, JD .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1999, 104 (D20) :24341-24357
[17]   Physical properties of stratospheric clouds during the Antarctic winter of 1995 [J].
Gobbi, GP ;
Di Donfrancesco, G ;
Adriani, A .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1998, 103 (D9) :10859-10873
[18]   LABORATORY STUDIES OF THE NITRIC-ACID TRIHYDRATE - IMPLICATIONS FOR THE SOUTH POLAR STRATOSPHERE [J].
HANSON, D ;
MAUERSBERGER, K .
GEOPHYSICAL RESEARCH LETTERS, 1988, 15 (08) :855-858
[19]  
Höpfner M, 2006, ATMOS CHEM PHYS, V6, P1201
[20]   Impact of polar stratospheric cloud particle composition, number density, and lifetime on denitrification [J].
Jensen, EJ ;
Toon, OB ;
Tabazadeh, A ;
Drdla, K .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2002, 107 (D20)