Iron phosphide as negative electrode material for Na-ion batteries

被引：90

作者：

Zhang, Wanjie ^{[1
]}

Dahbi, Mouad ^{[1
,2
]}

Amagasa, Shota ^{[1
]}

Yamada, Yasuhiro ^{[1
]}

Komaba, Shinichi ^{[1
,2
]}

机构：

[1] Tokyo Univ Sci, Shinjuku Ku, Tokyo 1628601, Japan

[2] Kyoto Univ, Elements Strategy Initiat Catalysts & Batteries, Kyoto 6158245, Japan

来源：

ELECTROCHEMISTRY COMMUNICATIONS | 2016年 / 69卷

关键词：

Na-ion battery; Negative electrode material; Conversion material; Transition metal phosphide; PROMISING ANODE MATERIAL; SODIUM-ION; HIGH-CAPACITY; LI; GRAPHITE; POLYACRYLATE; PERFORMANCE; STORAGE; MOSSBAUER; COMPOSITE;

D O I：

10.1016/j.elecom.2016.05.005

中图分类号：

O646 [电化学、电解、磁化学];

学科分类号：

081704 ;

摘要：

Iron phosphides, FeP2 and FeP4, have been synthesized and characterized for the application to non-aqueous Na-ion battery. FeP2 shows no significant electrochemical reactivity in Na-cell. However, FeP4 composite electrode with sodium polyacrylate binder delivers a reversible capacity of 1137 mAh.g(-1) and a Coulombic efficiency of 84.0% during the first cycle under a current density of 89 mA.g(-1). The high capacity is maintained for 30 cycles. Moreover, FeP4 composite electrode presents a good rate capability. Although the sodiation mechanism of FeP4 has not been fully understood, FeP4 is a new promising negative electrode material for Na-ion batteries with both high-power and high-energy densities. (C) 2016 Elsevier B.V. All rights reserved.

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页码：11 / 14

页数：4

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