Promotion effect of CuO co-catalyst on WO3-catalyzed photo degradation of organic substances

被引:87
作者
Arai, Takeo [1 ]
Yanagida, Masatoshi [1 ]
Konishi, Yoshinari [1 ]
Iwasaki, Yasukazu [2 ]
Sugihara, Hideki [1 ]
Sayama, Kazuhiro [1 ]
机构
[1] Nat Inst Adv Ind Sci & Technol AIST, Energy Technol Res Inst, Tsukuba, Ibaraki 3058565, Japan
[2] Nissan Motor Co Ltd, Nissan Res Ctr, Yokosuka, Kanagawa 2378523, Japan
关键词
D O I
10.1016/j.catcom.2007.11.012
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
CuO was found to be an effective co-catalyst for WO3-catalyzed photodegradation of acetaldehyde to CO2 under visible light. Loading CuO on WO3 also markedly promoted the photodegradation of other volatile organic compounds (VOCs), such as hexane, ethyl acetate, acetone, and diethyl ether. CuO appears to accelerate the oxygen-reduction process in the dark, and a reaction mechanism that the enhancement of reactivity was caused by this acceleration is proposed. (C) 2007 Elsevier B.V. All rights reserved.
引用
收藏
页码:1254 / 1258
页数:5
相关论文
共 17 条
[1]   Efficient complete oxidation of acetaldehyde into CO2 over CuBi2O4/WO3 composite photocatalyst under visible and UV light irradiation [J].
Arai, Takeo ;
Yanagida, Masatoshi ;
Konishi, Yoshinari ;
Iwasaki, Yasukazu ;
Sugihara, Hideki ;
Sayama, Kazuhiro .
JOURNAL OF PHYSICAL CHEMISTRY C, 2007, 111 (21) :7574-7577
[2]   Visible-light photocatalysis in nitrogen-doped titanium oxides [J].
Asahi, R ;
Morikawa, T ;
Ohwaki, T ;
Aoki, K ;
Taga, Y .
SCIENCE, 2001, 293 (5528) :269-271
[3]   PHOTOOXIDATION OF WATER SENSITIZED BY WO3 POWDER [J].
DARWENT, JR ;
MILLS, A .
JOURNAL OF THE CHEMICAL SOCIETY-FARADAY TRANSACTIONS II, 1982, 78 :359-367
[4]   Photocatalytic behavior of mixed WO3/WS2 powders [J].
Di Paola, A ;
Palmisano, L ;
Augugliaro, V .
CATALYSIS TODAY, 2000, 58 (2-3) :141-149
[5]   VISIBLE-LIGHT-INDUCED O-2 GENERATION FROM AQUEOUS DISPERSIONS OF WO3 [J].
ERBS, W ;
DESILVESTRO, J ;
BORGARELLO, E ;
GRATZEL, M .
JOURNAL OF PHYSICAL CHEMISTRY, 1984, 88 (18) :4001-4006
[6]   Photodegradation of toluene over TiO2-xNx under visible light irradiation [J].
Irokawa, Y ;
Morikawa, T ;
Aoki, K ;
Kosaka, S ;
Ohwaki, T ;
Taga, Y .
PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2006, 8 (09) :1116-1121
[7]   Highly active meso-microporous TaON photocatalyst driven by visible light [J].
Ito, S ;
Thampi, KR ;
Comte, P ;
Liska, P ;
Grätzel, M .
CHEMICAL COMMUNICATIONS, 2005, (02) :268-270
[8]   EFFECT OF INTERFACIAL PH ON THE REDUCTION OF OXYGEN ON COPPER IN NEUTRAL NACLO4 SOLUTION [J].
KING, F ;
LITKE, CD ;
TANG, Y .
JOURNAL OF ELECTROANALYTICAL CHEMISTRY, 1995, 384 (1-2) :105-113
[9]   Oxygen reduction in phosphate solution with the Cu(II) complex of 1,10-phenanthroline at glassy carbon electrode [J].
Liu, SJ ;
Huang, CH ;
Chang, CC .
MATERIALS CHEMISTRY AND PHYSICS, 2003, 82 (03) :551-556
[10]   PHOTOCATALYTIC DECOMPOSITION OF WATER AT SEMICONDUCTOR ELECTRODES [J].
MARUSKA, HP ;
GHOSH, AK .
SOLAR ENERGY, 1978, 20 (06) :443-458