Slow Magnetic Order-Order Transition in the Spin Chain Antiferromagnet Ca3Co2O6

被引:87
作者
Agrestini, S. [1 ,2 ]
Fleck, C. L. [3 ]
Chapon, L. C. [4 ]
Mazzoli, C. [5 ]
Bombardi, A. [6 ]
Lees, M. R. [3 ]
Petrenko, O. A. [3 ]
机构
[1] Lab CRISMAT, CNRS, UMR 6508, F-14050 Caen, France
[2] Max Planck Inst Chem Phys Solids, D-01187 Dresden, Germany
[3] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England
[4] Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England
[5] European Synchrotron Radiat Facil, F-38043 Grenoble 9, France
[6] Diamond Light Source Ltd, Rutherford Appleton Lab, Didcot OX11 0DE, Oxon, England
基金
英国工程与自然科学研究理事会;
关键词
ONE-DIMENSIONAL CA3CO2O6; CRYSTAL NEUTRON-DIFFRACTION; SINGLE-CRYSTAL; COMPOUND CA3CO2O6;
D O I
10.1103/PhysRevLett.106.197204
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Using powder neutron diffraction, we have discovered an unusual magnetic order-order transition in the Ising spin chain compound Ca3Co2O6. On lowering the temperature, an antiferromagnetic phase with a propagation vector k = (0.5, -0.5, 1) emerges from a higher temperature spin density wave structure with k = (0, 0, 1.01). This transition occurs over an unprecedented time scale of several hours and is never complete.
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页数:4
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