Ag2O nanoparticle/TiO2 nanobelt heterostructures with remarkable photo-response and photocatalytic properties under UV, visible and near-infrared irradiation

被引:223
作者
Wei, Na [1 ]
Cui, Hongzhi [1 ]
Song, Qiang [1 ]
Zhang, Liqiang [1 ]
Song, Xiaojie [1 ]
Wang, Ke [1 ]
Zhang, Yanfeng [1 ]
Li, Jian [1 ]
Wen, Jing [1 ]
Tian, Jian [1 ]
机构
[1] Shandong Univ Sci & Technol, Sch Mat Sci & Engn, Qingdao 266590, Peoples R China
基金
国家高技术研究发展计划(863计划); 中国国家自然科学基金;
关键词
Heterostructures; TiO2; nanobelt; Photocatalytic; UV-vis-NIR light; HIGHLY EFFICIENT; TITANIUM-DIOXIDE; DEGRADATION; FILM; NANOCOMPOSITES; AG2O/G-C3N4; COMPOSITES; ARRAYS; SILVER; OXIDE;
D O I
10.1016/j.apcatb.2016.05.040
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Finding a novel photocatalyst that can operate over a broad range of wavelengths from UV to near-infrared (NIR) holds great potential for diverse uses. Here, an Ag2O nanoparticle/TiO2 nanobelt heterostructure with enhanced photocatalytic performance of degrading methyl orange (MO) under UV, visible and NIR irradiation is prepared. Such an excellent photocatalytic performance is ascribed to the synergistic effects, including highly dispersed Ag2O nanoparticles on the surface of TiO2 nanobelts and efficient charge separation efficiency induced by the heterostructure between Ag2O and TiO2. Finally, a possible photocatalytic mechanism is proposed for this novel photocatalyst. This current work can afford a new paradigm for the full utilization of solar light. (C) 2016 Elsevier B.V. All rights reserved.
引用
收藏
页码:83 / 90
页数:8
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