Electrogenerated Chemiluminescence of Au Nanoclusters for the Detection of Dopamine

被引：348

作者：

Li, Lingling ^{[1
]}

Liu, Hongying ^{[1
]}

Shen, Yuanyuan ^{[1
]}

Zhang, Jianrong ^{[1
]}

Zhu, Jun-Jie ^{[1
]}

机构：

[1] Nanjing Univ, Key Lab Analyt Chem Life Sci, Minist Educ China, Sch Chem & Chem Engn, Nanjing 210093, Peoples R China

来源：

ANALYTICAL CHEMISTRY | 2011年 / 83卷 / 03期

基金：

中国国家自然科学基金;

关键词：

FLUORESCENT GOLD NANOCLUSTERS; QUANTUM DOTS; ELECTROCHEMILUMINESCENCE; CLUSTERS; ELECTROCHEMISTRY; NANOCRYSTALS; STATE; TIO2;

D O I：

10.1021/ac102623r

中图分类号：

O65 [分析化学];

学科分类号：

070302 ; 081704 ;

摘要：

Electrogenerated chemiluminescence (ECL) emission was observed from the water-soluble, bovine serum albumin (BSA)-stabilized Au nanoclusters for the first time. The possible ECL mechanism was discussed according to the presented results and ascribed to the effective electron transfer from the conduction-band of excited indium tin oxide (ITO) to Au nanoclusters (NCs). A simple label-free method for the detection of dopamine has been developed based on the Au NCs ECL in aqueous media The Au NCs could be an effective candidate for new types of ECL biosensors in the future due to their fascinating features, such as good water solubility, low toxicity, ease of labeling, and excellent stability.

引用

收藏

页码：661 / 665

页数：5

相关论文

共 27 条

[1] Electrochemistry and electrogenerated chemiluminescence of films of silicon nanoparticles in aqueous solution [J].

Bae, Yoonjung ;

Lee, Doh C. ;

Rhogojina, Elena V. ;

Jurbergs, David C. ;

Korgel, Brian A. ;

Bard, Allen J. .

NANOTECHNOLOGY, 2006, 17 (15) :3791-3797

[2] Color Tunability and Electrochemiluminescence of Silver Nanoclusters [J].

Diez, Isabel ;

Pusa, Matti ;

Kulmala, Sakari ;

Jiang, Hua ;

Walther, Andreas ;

Goldmann, Anja S. ;

Muller, Axel H. E. ;

Ikkala, Olli ;

Ras, Robin H. A. .

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2009, 48 (12) :2122-2125

[3] Enhanced solid-state electrochemiluminescence of CdS nanocrystals composited with carbon nanotubes in H2O2 solution [J].

Ding, Shou-Nian ;

Xu, Jing-Juan ;

Chen, Hong-Yuan .

CHEMICAL COMMUNICATIONS, 2006, (34) :3631-3633

[4] Electrochemistry and electrogenerated chemiluminescence from silicon nanocrystal quantum dots [J].

Ding, ZF ;

Quinn, BM ;

Haram, SK ;

Pell, LE ;

Korgel, BA ;

Bard, AJ .

SCIENCE, 2002, 296 (5571) :1293-1297

[5] Enhanced quantum yield of dendrimer-entrapped gold nanodots by a specific ion-pair association and microwave irradiation for bioimaging [J].

Jao, Yu-Chen ;

Chen, Meng-Kai ;

Lin, Shu-Yi .

CHEMICAL COMMUNICATIONS, 2010, 46 (15) :2626-2628

[6] Electrochemiluminescence immunosensor based on CdSe nanocomposites [J].

Jie, Guifen ;

Zhang, Jingjing ;

Wang, Danchen ;

Cheng, Chao ;

Chen, Hong-Yuan ;

Zhu, Jun-Jie .

ANALYTICAL CHEMISTRY, 2008, 80 (11) :4033-4039

[7] CdS nanocrystal-based electrochemiluminescence biosensor for the detection of low-density lipoprotein by increasing sensitivity with gold nanoparticle amplification [J].

Jie, Guifen ;

Liu, Bo ;

Pan, Hongcheng ;

Zhu, Jun-Jie ;

Chen, Hong-Yuan .

ANALYTICAL CHEMISTRY, 2007, 79 (15) :5574-5581

[8] Quantum sized, thiolate-protected gold nanoclusters [J].

Jin, Rongchao .

NANOSCALE, 2010, 2 (03) :343-362

[9] Suppressed Blinking Dynamics of Single QDs on ITO [J].

Jin, Shengye ;

Song, Nianhui ;

Lian, Tianquan .

ACS NANO, 2010, 4 (03) :1545-1552

[10] Size-controlled interparticle charge transfer between TiO2 and quantized capacitors [J].

Kim, Junhyung ;

Lee, Dongil .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2007, 129 (25) :7706-+