Processing of mussel-adhesive protein analog copolymer thin films by matrix-assisted pulsed laser evaporation

被引:14
作者
Patz, T
Cristescu, R
Narayan, R
Menegazzo, N
Mizaikoff, B
Messersmith, PB
Stamatin, I
Mihailescu, L
Chrisey, DB
机构
[1] Natl Inst Lasers Plasma & Radiat Phys, RO-077125 Bucharest, Romania
[2] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA
[3] Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA
[4] Northwestern Univ, Dept Biomed Engn, Robert R McCormick Sch Engn & Appl Sci, Evanston, IL 60208 USA
[5] USN, Res Lab, Washington, DC 20375 USA
[6] Univ Bucharest, Fac Phys, Bucharest, Romania
关键词
mussel-adhesive protein; matrix-assisted pulsed laser evaporation;
D O I
10.1016/j.apsusc.2005.03.056
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We have demonstrated the successful thin film growth of a mussel-adhesive protein analog, DOPA-modified PEO-PPO-PEO block copolymer PF127, using matrix-assisted pulsed laser evaporation (MAPLE). The MAPLE-deposited thin films were examined using Fourier transform infrared spectroscopy, atomic force microscopy, X-ray photoelectron spectroscopy, and contact-angle measurements. We have found that the main functional groups of the mussel-adhesive protein analog are present in the transferred film. These adhesive materials have several potential electronic, medical, and marine applications. (c) 2005 Elsevier B.V. All rights reserved.
引用
收藏
页码:416 / 421
页数:6
相关论文
共 24 条
[1]  
[Anonymous], 1998, SURG ADHESIVES SEALA
[2]   Adsorption of adhesive proteins from the marine mussel, Mytilus edulis, on polymer films in the hydrated state using angle dependent X-ray photoelectron spectroscopy and atomic force microscopy [J].
Baty, AM ;
Leavitt, PK ;
Siedlecki, CA ;
Tyler, BJ ;
Suci, PA ;
Marchant, RE ;
Geesey, GG .
LANGMUIR, 1997, 13 (21) :5702-5710
[3]   Environmental bioadhesion: Themes and applications [J].
Burzio, LO ;
Burzio, VA ;
Silva, T ;
Burzio, LA ;
Pardo, J .
CURRENT OPINION IN BIOTECHNOLOGY, 1997, 8 (03) :309-312
[4]   Laser deposition of polymer and biomaterial films [J].
Chrisey, DB ;
Piqué, A ;
McGill, RA ;
Horwitz, JS ;
Ringeisen, BR ;
Bubb, DM ;
Wu, PK .
CHEMICAL REVIEWS, 2003, 103 (02) :553-576
[5]   Materials science of adhesives: How to bond things together [J].
Creton, C ;
Papon, E .
MRS BULLETIN, 2003, 28 (06) :419-421
[6]   Polymer reptation in disordered media [J].
Cule, D ;
Hwa, T .
PHYSICAL REVIEW LETTERS, 1998, 80 (14) :3145-3148
[7]  
Harding SE, 2003, BIOCHEM SOC T, V31, P1036
[8]   Synthesis and characterization of self-assembling block copolymers containing bioadhesive end groups [J].
Huang, K ;
Lee, BP ;
Ingram, DR ;
Messersmith, PB .
BIOMACROMOLECULES, 2002, 3 (02) :397-406
[9]   Synthesis and gelation of DOPA-Modified poly(ethylene glycol) hydrogels [J].
Lee, BP ;
Dalsin, JL ;
Messersmith, PB .
BIOMACROMOLECULES, 2002, 3 (05) :1038-1047
[10]  
Lin-Vien D., 1991, The Handbook of Infrared and Raman Characteristic Frequencies of Organic Molecules