A highly stable MnII phosphonate as a highly efficient catalyst for CO2 fixation under ambient conditions

被引：44

作者：

Yang, Yang ^{[1
]}

Gao, Chao-Ying ^{[1
,2
]}

Tian, Hong-Rui ^{[2
]}

Ai, Jing ^{[2
]}

Min, Xue ^{[2
]}

Sun, Zhong-Ming ^{[2
]}

机构：

[1] IMUN, Coll Chem & Chem Engn, Inner Mongolia Key Lab Chem Nat Prod & Synth Func, Tongliao 028000, Peoples R China

[2] Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Rare Earth Resource Utilizat, 5625 Renmin St, Changchun 130022, Jilin, Peoples R China

来源：

CHEMICAL COMMUNICATIONS | 2018年 / 54卷 / 14期

基金：

中国国家自然科学基金;

关键词：

METAL-ORGANIC FRAMEWORKS; CARBON-DIOXIDE CAPTURE; CYCLIC CARBONATES; POLYMER NETWORKS; SELECTIVE CO2; EPOXIDES; CYCLOADDITION; ADSORPTION; CONVERSION; DESIGN;

D O I：

10.1039/c7cc09867g

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

With coordinatively unsaturated metal centers decorating the channel walls, a Mn-II phosphonate exhibits highly efficient and substrate size-selective catalysis in the context of CO2 chemical conversion into cyclic carbonates under 1 atm pressure and at room temperature, proving to be a promising heterogeneous catalyst in an eco-friendly and energy efficient way.

引用

页码：1758 / 1761

页数：4

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