Proximity-Induced Gap Opening by Twisted Plumbene in Epitaxial Graphene

被引:24
作者
Ghosal, Chitran [1 ]
Gruschwitz, Markus [1 ]
Koch, Julian [1 ]
Gemming, Sibylle [1 ]
Tegenkamp, Christoph [1 ]
机构
[1] Tech Univ Chemnitz, Inst Phys, Reichenhainer Str 70, D-09126 Chemnitz, Germany
关键词
D O I
10.1103/PhysRevLett.129.116802
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Besides graphene, further honeycomb 2D structures were successfully synthesized on various surfaces. However, almost flat plumbene hosting topologically protected edge states could not yet be realized. In this Letter, we investigated the intercalation of Pb on buffer layers on SiC(0001). Thereby, suspended and charge neutral graphene emerged, and the intercalated Pb formed plumbene honeycomb lattices, which are rotated by & PLUSMN;7.5 & DEG; with respect to graphene. Along with this twist, a proximity-induced modulation of the hopping parameter in graphene opens a band gap of around 30 meV at the Fermi energy, giving rise to a metal-insulator transition. Moreover, the edges of the intercalated plumbene layers revealed edge states within the gap of the conduction bands at around 1 eV as expected for charge neutral plumbene.
引用
收藏
页数:6
相关论文
共 34 条
[1]   Germanene termination of Ge2Pt crystals on Ge(110) [J].
Bampoulis, P. ;
Zhang, L. ;
Safaei, A. ;
van Gastel, R. ;
Poelsema, B. ;
Zandvliet, H. J. W. .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2014, 26 (44)
[2]   Design and realization of topological Dirac fermions on a triangular lattice [J].
Bauernfeind, Maximilian ;
Erhardt, Jonas ;
Eck, Philipp ;
Thakur, Pardeep K. ;
Gabel, Judith ;
Lee, Tien-Lin ;
Schaefer, Joerg ;
Moser, Simon ;
Di Sante, Domenico ;
Claessen, Ralph ;
Sangiovanni, Giorgio .
NATURE COMMUNICATIONS, 2021, 12 (01)
[3]   Plumbene on a Magnetic Substrate: A Combined Scanning Tunneling Microscopy and Density Functional Theory Study [J].
Bihlmayer, Gustav ;
Sassmannshausen, Jonas ;
Kubetzka, Andre ;
Bluegel, Stefan ;
von Bergmann, Kirsten ;
Wiesendanger, Roland .
PHYSICAL REVIEW LETTERS, 2020, 124 (12)
[4]  
Calleja F, 2015, NAT PHYS, V11, P43, DOI [10.1038/nphys3173, 10.1038/NPHYS3173]
[5]   Unconventional superconductivity in magic-angle graphene superlattices [J].
Cao, Yuan ;
Fatemi, Valla ;
Fang, Shiang ;
Watanabe, Kenji ;
Taniguchi, Takashi ;
Kaxiras, Efthimios ;
Jarillo-Herrero, Pablo .
NATURE, 2018, 556 (7699) :43-+
[6]   Silicene growth on Ag(110) and Ag(111) substrates reconsidered in light of Si-Ag reactivity [J].
Colonna, S. ;
Flammini, R. ;
Ronci, F. .
NANOTECHNOLOGY, 2021, 32 (15)
[7]   Growth of graphene on Ir(111) (vol 11, art no 023006, 2009) [J].
Coraux, Johann ;
N'Diaye, Alpha T. ;
Engler, Martin ;
Busse, Carsten ;
Wall, Dirk ;
Buckanie, Niemma ;
Heringdorf, Frank-J Meyer zu ;
van Gastel, Raoul ;
Poelsema, Bene ;
Michely, Thomas .
NEW JOURNAL OF PHYSICS, 2009, 11
[8]  
Emtsev KV, 2009, NAT MATER, V8, P203, DOI [10.1038/NMAT2382, 10.1038/nmat2382]
[9]  
Feng BJ, 2016, NAT CHEM, V8, P564, DOI [10.1038/nchem.2491, 10.1038/NCHEM.2491]
[10]   The rise of graphene [J].
Geim, A. K. ;
Novoselov, K. S. .
NATURE MATERIALS, 2007, 6 (03) :183-191