Applicability of the electrocoagulation process in treating real municipal wastewater containing pharmaceutical active compounds

被引：86

作者：

Ensano, Benny Marie B. ^{[1
]}

Borea, Laura ^{[2
]}

Naddeo, Vincenzo ^{[2
]}

Belgiorno, Vincenzo ^{[2
]}

de Luna, Mark Daniel G. ^{[1
,3
]}

Balakrishnan, Malini ^{[4
]}

Ballesteros, Florencio C., Jr. ^{[1
,3
]}

机构：

[1] Univ Philippines, Natl Grad Sch Engn, Environm Engn Program, Quezon City 1101, Philippines

[2] Univ Salerno, Dept Civil Engn, SEED, I-84084 Fisciano, SA, Italy

[3] Univ Philippines, Dept Chem Engn, Quezon City 1101, Philippines

[4] India Habitat Ctr, Energy & Resources Inst TERI, Darbari Seth Block,Lodi Rd, New Delhi 110003, India

来源：

JOURNAL OF HAZARDOUS MATERIALS | 2019年 / 361卷

关键词：

Amoxicillin; Carbamazepine; Diclofenac; Electrochemical processes; Emerging contaminants; REMOVAL; OPTIMIZATION; BIOACCUMULATION; CONTAMINANTS; COAGULATION; GROUNDWATER; OXIDATION; NUTRIENT;

D O I：

10.1016/j.jhazmat.2018.07.093

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

In this study, the viability of using electrocoagulation process as a method for pharmaceuticals removal from real municipal wastewater was demonstrated. Batch experimental runs were performed using a simple laboratory scale electrochemical reactor with aluminium and stainless steel as anode and cathode, respectively. Diclofenac (DCF), carbamazepine (CBZ) and amoxicillin (AMX) were selected as representative of pharmaceuticals frequently detected in the aquatic environment. The effects of varying experimental parameters namely current density (0.3, 0.5 1.15 and 1.8 mA cm(-2)), initial pharmaceutical concentration (0.01, 4 and 10 mg L-1), electrolysis duration (3, 6 and 19 h) and application mode (continuous vs. intermittent) on pharmaceutical removal efficiencies were evaluated. High pharmaceutical abatement was recorded at elevated current density and prolonged electrolysis duration due to additional electro-generated coagulant species in solution.

引用

页码：367 / 373

页数：7

共 39 条

[1] Micropollutants removal from retentates generated in ultrafiltration and nanofiltration treatments of municipal secondary effluents by means of coagulation, oxidation, and adsorption processes [J].

Acero, Juan L. ;

Javier Benitez, F. ;

Real, Francisco J. ;

Teva, Fernando .

CHEMICAL ENGINEERING JOURNAL, 2016, 289 :48-58

[2]

APAT IRSA-CNR, 2003, MET AN ACQ MAN LIN G

[3] Integrated treatment of molasses distillery wastewater using microfiltration (MF) [J].

Basu, Subhankar ;

Mukherjee, Sangeeta ;

Kaushik, Ankita ;

Batra, Vidya S. ;

Balakrishnan, Malini .

JOURNAL OF ENVIRONMENTAL MANAGEMENT, 2015, 158 :55-60

[4] Treatment of the textile wastewater by combined electrocoagulation [J].

Can, OT ;

Kobya, M ;

Demirbas, E ;

Bayramoglu, M .

CHEMOSPHERE, 2006, 62 (02) :181-187

[5] Treatment of highly concentrated tannery wastewater using electrocoagulation: Influence of the quality of aluminium used for the electrode [J].

Elabbas, S. ;

Ouazzani, N. ;

Mandi, L. ;

Berrekhis, F. ;

Perdicakis, M. ;

Pontvianne, S. ;

Pons, M-N. ;

Lapicque, F. ;

Leclerc, J-P .

JOURNAL OF HAZARDOUS MATERIALS, 2016, 319 :69-77

[6] Combination of Electrochemical Processes with Membrane Bioreactors for Wastewater Treatment and Fouling Control: A Review [J].

Ensano, Benny M. B. ;

Borea, Laura ;

Naddeo, Vincenzo ;

Belgiorno, Vincenzo ;

de Luna, Mark D. G. ;

Ballesteros, Florencio C., Jr. .

FRONTIERS IN ENVIRONMENTAL SCIENCE, 2016, 4

[7] Control of emerging contaminants by the combination of electrochemical processes and membrane bioreactors [J].

Ensano, Benny Marie B. ;

Borea, Laura ;

Naddeo, Vincenzo ;

de Luna, Mark Daniel G. ;

Belgiorno, Vincenzo .

ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH, 2019, 26 (02) :1103-1112

[8] Removal of Pharmaceuticals from Wastewater by Intermittent Electrocoagulation [J].

Ensano, Benny Marie B. ;

Borea, Laura ;

Naddeo, Vincenzo ;

Belgiorno, Vincenzo ;

de Luna, Mark Daniel G. ;

Ballesteros, Florencio C., Jr. .

WATER, 2017, 9 (02)

[9] Electrochemical advanced oxidation and biological processes for wastewater treatment: a review of the combined approaches [J].

Ganzenko, Oleksandra ;

Huguenot, David ;

van Hullebusch, Eric D. ;

Esposito, Giovanni ;

Oturan, Mehmet A. .

ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH, 2014, 21 (14) :8493-8524

[10] Optimization of electrocoagulation (EC) process for the purification of a real industrial wastewater from toxic metals [J].

Gatsios, Evangelos ;

Hahladakis, John N. ;

Gidarakos, Evangelos .

JOURNAL OF ENVIRONMENTAL MANAGEMENT, 2015, 154 :117-127

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