Synthesis of furoic acid from biomass via tandem pretreatment and biocatalysis

被引：35
作者：
Yang, Dong [1 ]
Ma, Cuiluan [2 ]
Peng, Bo [2 ]
Xu, Jianhe [3 ]
He, Yu-Cai [1 ,2 ,3 ]
机构：
[1] Changzhou Univ, Natl Local Joint Engn Res Ctr Biomass Refining &, Adv Catalysis & Green Mfg Collaborat Innovat Ctr, Jiangsu Key Lab Adv Catalyt Mat & Technol,Sch Pha, Changzhou 213164, Peoples R China
[2] Hubei Univ, Sch Life Sci, Hubei Key Lab Ind Biotechnol, State Key Lab Biocatalysis & Enzyme Engn,Hubei Co, Wuhan 430062, Peoples R China
[3] East China Univ Sci & Technol, Shanghai Collaborat Innovat Ctr Biomfg, State Key Lab Bioreactor Engn, Shanghai 200237, Peoples R China
来源：
INDUSTRIAL CROPS AND PRODUCTS | 2020年 / 153卷
基金：
中国国家自然科学基金;
关键词：
Sn-adamellite; Bamboo shoot shell; Furfural; Furoic acid; Biocatalysis; LIGNOCELLULOSIC BIOMASS; IONIC LIQUIDS; ETHANOL; XYLOSE; HYDROLYSATE; OXIDATION; ALDEHYDES; ZEOLITE;
D O I：
10.1016/j.indcrop.2020.112580
中图分类号：
S2 [农业工程];
学科分类号：
0828 ;
摘要：
Upgradation of bio-based product furfural into important intermediates is of great interest. In this study, tinbased adamellite (Sn-adamellite) was firstly synthesized for converting bamboo shoot shell (BSS) into furfural. The optimum solid acid Sn-adamellite loading, pretreatment temperature and pretreatment time were 3.0 wt%, 170 degrees C and 30 min, respectively. SEM and FT-IR images and chemical components of untreated and pretreated BSS samples indicated that sequential alkalic soaking and solid acid pretreatment could be effectively used for removing xylan in biomass. Furthermore, recombinant E. coli BH harboring horse liver alcohol dehydrogenase (HLADH) was constructed for the biotransformation of 30 mM furfural into furoic acid with 100% analytical yield at pH 7.5 and 35 degrees C. Finally, an effective hybrid strategy was successfully developed for converting BSS to furoic acid by tandem catalysis via Sn-adamellite pretreatment combined with recombinant E. coli whole cells harboring HLADH.
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页数：7
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