A monolithic metal-free electrocatalyst for oxygen evolution reaction and overall water splitting

被引：188

作者：

Balogun, Muhammad-Sadeeq ^{[1
]}

Qiu, Weitao ^{[1
]}

Yang, Hao ^{[1
]}

Fan, Wenjie ^{[1
]}

Huang, Yongchao ^{[1
]}

Fang, Pingping ^{[1
]}

Li, Gaoren ^{[1
]}

Ji, Hongbing ^{[1
]}

Tong, Yexiang ^{[1
]}

机构：

[1] Sun Yat Sen Univ, Sch Chem, KLGHEI Environm & Energy Chem, MOE Key Lab Bioinorgan & Synthet Chem,Key Lab Low, 135 Xingang West Rd, Guangzhou 510275, Guangdong, Peoples R China

来源：

ENERGY & ENVIRONMENTAL SCIENCE | 2016年 / 9卷 / 11期

关键词：

CARBON-FIBER CLOTH; HIGHLY EFFICIENT; ENERGY-CONVERSION; NITROGEN; ARRAYS; OXIDATION; REDUCTION; HYDROGEN; EXFOLIATION; COMPOSITES;

D O I：

10.1039/c6ee01930g

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Herein, a three-dimensional monolithic and metal-free N-doped porous carbon cloth electrocatalyst was fabricated. Owing to the increased surface area and N-doping, the self-supporting electrocatalyst could effectively catalyze the oxygen evolution reaction, and was also utilized as the anode for an alkaline electrolyzer for the first time with a considerably low overpotential.

引用

页码：3411 / 3416

页数：6

共 36 条

[1] All-flexible lithium ion battery based on thermally-etched porous carbon cloth anode and cathode [J].

Balogun, Muhammad-Sadeeq ;

Qiu, Weitao ;

Lyu, Feiyi ;

Luo, Yang ;

Meng, Hui ;

Li, Jiantao ;

Mai, Wenjie ;

Mai, Liqiang ;

Tong, Yexiang .

NANO ENERGY, 2016, 26 :446-455

[2] Iridium Oxide Coatings with Templated Porosity as Highly Active Oxygen Evolution Catalysts: Structure-Activity Relationships [J].

Bernicke, Michael ;

Ortel, Erik ;

Reier, Tobias ;

Bergmann, Arno ;

de Araujo, Jorge Ferreira ;

Strasser, Peter ;

Kraehnert, Ralph .

CHEMSUSCHEM, 2015, 8 (11) :1908-1915

[3] Paper-Based N-Doped Carbon Films for Enhanced Oxygen Evolution Electrocatalysis [J].

Chen, Sheng ;

Duan, Jingjing ;

Ran, Jinrun ;

Qiao, Shi-Zhang .

ADVANCED SCIENCE, 2015, 2 (1-2)

[4] Nitrogen and Oxygen Dual-Doped Carbon Hydrogel Film as a Substrate-Free Electrode for Highly Efficient Oxygen Evolution Reaction [J].

Chen, Sheng ;

Duan, Jingjing ;

Jaroniec, Mietek ;

Qiao, Shi-Zhang .

ADVANCED MATERIALS, 2014, 26 (18) :2925-2930

[5] Three-Dimensional N-Doped Graphene Hydrogel/NiCo Double Hydroxide Electrocatalysts for Highly Efficient Oxygen Evolution [J].

Chen, Sheng ;

Duan, Jingjing ;

Jaroniec, Mietek ;

Qiao, Shi Zhang .

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2013, 52 (51) :13567-13570

[6] N-doped graphene film-confined nickel nanoparticles as a highly efficient three-dimensional oxygen evolution electrocatalyst [J].

Chen, Sheng ;

Duan, Jingjing ;

Ran, Jingrun ;

Jaroniec, Mietek ;

Qiao, Shi Zhang .

ENERGY & ENVIRONMENTAL SCIENCE, 2013, 6 (12) :3693-3699

[7] Acidically oxidized carbon cloth: a novel metal-free oxygen evolution electrode with high catalytic activity [J].

Cheng, Ningyan ;

Liu, Qian ;

Tian, Jingqi ;

Xue, Yurui ;

Asiri, Abdullah M. ;

Jiang, Hongfang ;

He, Yuquan ;

Sun, Xuping .

CHEMICAL COMMUNICATIONS, 2015, 51 (09) :1616-1619

[8]

Feng J.-X., 2016, ANGEW CHEM, V128, P3758, DOI DOI 10.1002/ANGE.201511447

[9] Design and Synthesis of FeOOH/CeO2 Heterolayered Nanotube Electrocatalysts for the Oxygen Evolution Reaction [J].

Feng, Jin-Xian ;

Ye, Sheng-Hua ;

Xu, Han ;

Tong, Ye-Xiang ;

Li, Gao-Ren .

ADVANCED MATERIALS, 2016, 28 (23) :4698-4703

[10] High-Index Faceted Ni3S2 Nanosheet Arrays as Highly Active and Ultrastable Electrocatalysts for Water Splitting [J].

Feng, Liang-Liang ;

Yu, Guangtao ;

Wu, Yuanyuan ;

Li, Guo-Dong ;

Li, Hui ;

Sun, Yuanhui ;

Asefa, Tewodros ;

Chen, Wei ;

Zou, Xiaoxin .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2015, 137 (44) :14023-14026

← 1 2 3 4 →