Construction of 2D porphyrin-based covalent organic framework as adsorbent for organic dyes removal and carbon dioxide adsorption

被引：41
作者：
Chang, Siqi [1 ]
Xie, Wei [1 ]
Yao, Chan [1 ]
Xu, Guangjuan [1 ]
Zhang, Shuran [1 ]
Xu, Yanhong [1 ,2 ]
Ding, Xuesong [3 ]
机构：
[1] Jilin Normal Univ, Key Lab Preparat & Applicat Environm Friendly Mat, Key Lab Funct Mat Phys & Chem, Minist Educ, Changchun 130103, Peoples R China
[2] Changchun Univ Sci & Technol, Collaborat Innovat Ctr Opt Mat & Chem, Sch Sch Chem & Environm Engn, Changchun 130022, Peoples R China
[3] Natl Ctr Nanosci & Technol, CAS Ctr Excellence Nanosci, CAS Key Lab Nanosyst & Hierarch Fabricat, Beijing 100190, Peoples R China
来源：
JOURNAL OF SOLID STATE CHEMISTRY | 2021年 / 304卷 / 304期
基金：
中国国家自然科学基金;
关键词：
2D covalent organic framework; Porphyrin; Tetraphenylethylene derivatives; Dye adsorption; Water treatment; NANOCOMPOSITES;
D O I：
10.1016/j.jssc.2021.122577
中图分类号：
O61 [无机化学];
学科分类号：
070301 ; 081704 ;
摘要：
A porphyrin-based two-dimensional covalent organic framework (TPE-Por-COF) with high stability was synthesized, and the adsorption performance of TPE-Por-COF on organic dyes was studied. The TPE-Por-COF was characterized by X-ray powder diffraction, infrared spectroscopy, solid-state nuclear magnetic resonance, thermogravimetry and N-2 adsorption isotherms. TPE-Por-COF has adsorption effect on five dyes: malachite green (MG), methyl violet (MV) and rhodamine B (RhB), coomassie brilliant blue (CBB) and brilliant green (BG). Among them, TPE-Por-COF has the most obvious adsorption effect on malachite green, and the adsorption capacity is as high as 1428.57 mg g(-1). In addition, the CO2 adsorption capacity of TPE-Por-COF is 187 mg g-1 at 50 bar and 323 K.
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页数：7
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