Determination of the mean aerosol residence times in the atmosphere and additional 210Po input on the base of simultaneous determination of 7Be, 22Na, 210Pb, 210Bi and 210Po in urban air

被引:26
作者
Dlugosz-Lisiecka, Magdalena [1 ]
Bem, Henryk [1 ]
机构
[1] Tech Univ Lodz, Inst Appl Radiat Chem, PL-90924 Lodz, Poland
关键词
Radionuclides; Aerosols; Residence time; TROPOSPHERIC AEROSOLS; ASSOCIATION; PROFILES; RN-222; CITY; LODZ;
D O I
10.1007/s10967-012-1690-5
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
The significant differences in the activities of Pb-210, Bi-210, Po-210 and cosmogenic Be-7 and Na-22 radionuclides in the urban aerosol samples collected in the summers 2010 and 2011 in the Lodz city of Poland were observed. Simultaneous measurement of these radionuclides, after a simple modification of the one compartment model, allows us to calculate both: the corrected aerosol residence times in the troposphere (1 A center dot 25 days) and in the lower stratosphere (103 A center dot 205 days). The relative input of the additional sources (beside of the Rn-222 decay in the air) to the total activity concentrations of Pb-210, Bi-210 and Po-210 radionuclides in the urban air, plays a substantial role (up to 97% of the total activity) only in the case of Po-210.
引用
收藏
页码:135 / 140
页数:6
相关论文
共 24 条
[2]   Residence time of arctic haze aerosols using the concentrations and activity ratios of 210Po, 210Pb and 7Be [J].
Baskaran, M ;
Shaw, GE .
JOURNAL OF AEROSOL SCIENCE, 2001, 32 (04) :443-452
[3]   ORIGINS AND CONCENTRATIONS OF RN-222, PB-210, BI-210 AND PO-210 IN THE SURFACE AIR AT LISBON, PORTUGAL, AT THE ATLANTIC EDGE OF THE EUROPEAN CONTINENTAL LANDMASS [J].
CARVALHO, FP .
ATMOSPHERIC ENVIRONMENT, 1995, 29 (15) :1809-1819
[4]  
Chamberlain AC, 1991, RADIOACTIVE AEROSOLS, P48
[5]   International recommendations offered on analytical detection and quantification concepts and nomenclature [J].
Currie, LA .
ANALYTICA CHIMICA ACTA, 1999, 391 (02) :103-103
[6]   210Pb and 210Po radionuclides in the urban air of Lodz, Poland [J].
Dlugosz, Magdalena ;
Grabowski, Pawel ;
Bem, Henryk .
JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY, 2010, 283 (03) :719-725
[7]  
Gaggeler HW, 1995, RADIOCHIM ACTA, V70-1, P345
[8]  
Grabowski P, 2010, NUKLEONIKA, V55, P181
[9]   Evidence for anthropogenic 210Po in the urban atmosphere of Seoul, Korea [J].
Kim, G ;
Hong, YL ;
Jang, J ;
Lee, I ;
Hwang, DW ;
Yang, HS .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2005, 39 (06) :1519-1522
[10]   Excess 210Po in the coastal atmosphere [J].
Kim, G ;
Hussain, N ;
Church, TM .
TELLUS SERIES B-CHEMICAL AND PHYSICAL METEOROLOGY, 2000, 52 (01) :74-80