Bio-inspired transparent MXene electrodes for flexible UV photodetectors

被引:158
|
作者
Chen, Jiaxin [1 ]
Li, Ziliang [1 ]
Ni, Fenglou [1 ]
Ouyang, Weixin [1 ]
Fang, Xiaosheng [1 ]
机构
[1] Fudan Univ, Dept Mat Sci, Shanghai 200438, Peoples R China
基金
国家重点研发计划; 中国国家自然科学基金;
关键词
RUTILE;
D O I
10.1039/d0mh00394h
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
2D transition metal carbides (MXenes) have emerged as one of the representative materials for transparent electrodes of electronics, but it is still a challenge to achieve highly transparent and conductive MXene electrodes for flexible photodetectors due to the tradeoff between resistance and transmittance. Herein, we put forward a bio-inspired transparent MXene film with a high transmittance of about 90% and low sheet resistance value of around 3 omega sq(-1). Moreover, thanks to the presence of various surface terminal groups, the MXene electrode's work function is adjustableviadifferent etching processes, and in conjunction with electrospun TiO(2)films a semi-transparent UV photodetector is integrated. Furthermore, the electrode and the constructed photodetector both exhibit superb flexibility which can survive 1000 bending cycles. This work not only provides a novel pathway to simultaneously improve the transmittance and conductivity of transparent electrodes, but also is available for extensive applications of optoelectronics.
引用
收藏
页码:1828 / 1833
页数:6
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