Significant atmospheric aerosol pollution caused by world food cultivation

被引:160
作者
Bauer, Susanne E. [1 ,2 ]
Tsigaridis, Kostas [1 ,2 ]
Miller, Ron [2 ,3 ,4 ]
机构
[1] Columbia Univ, Earth Inst, Ctr Climate Syst Res, New York, NY USA
[2] NASA, Goddard Inst Space Studies, New York, NY 10025 USA
[3] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY USA
[4] Columbia Univ, Dept Earth & Environm Sci, New York, NY USA
关键词
PARTICULATE MATTER; NITROGEN-CYCLE; AIR-QUALITY; EMISSIONS; AGRICULTURE; MORTALITY; GASES;
D O I
10.1002/2016GL068354
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
Particulate matter is a major concern for public health, causing cancer and cardiopulmonary mortality. Therefore, governments in most industrialized countries monitor and set limits for particulate matter. To assist policy makers, it is important to connect the chemical composition and severity of particulate pollution to its sources. Here we show how agricultural practices, livestock production, and the use of nitrogen fertilizers impact near-surface air quality. In many densely populated areas, aerosols formed from gases that are released by fertilizer application and animal husbandry dominate over the combined contributions from all other anthropogenic pollution. Here we test reduction scenarios of combustion-based and agricultural emissions that could lower air pollution. For a future scenario, we find opposite trends, decreasing nitrate aerosol formation near the surface while total tropospheric loads increase. This suggests that food production could be increased to match the growing global population without sacrificing air quality if combustion emission is decreased.
引用
收藏
页码:5394 / 5400
页数:7
相关论文
共 29 条
[1]   Effects of Agriculture upon the Air Quality and Climate: Research, Policy, and Regulations [J].
Aneja, Viney P. ;
Schlesinger, William H. ;
Erisman, Jan Willem .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2009, 43 (12) :4234-4240
[2]   MATRIX (Multiconfiguration Aerosol TRacker of mIXing state): an aerosol microphysical module for global atmospheric models [J].
Bauer, S. E. ;
Wright, D. L. ;
Koch, D. ;
Lewis, E. R. ;
McGraw, R. ;
Chang, L. -S. ;
Schwartz, S. E. ;
Ruedy, R. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2008, 8 (20) :6003-6035
[3]   Nitrate aerosols today and in 2030: a global simulation including aerosols and tropospheric ozone [J].
Bauer, S. E. ;
Koch, D. ;
Unger, N. ;
Metzger, S. M. ;
Shindell, D. T. ;
Streets, D. G. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2007, 7 (19) :5043-5059
[4]   Impact of the modal aerosol scheme GLOMAP-mode on aerosol forcing in the Hadley Centre Global Environmental Model [J].
Bellouin, N. ;
Mann, G. W. ;
Woodhouse, M. T. ;
Johnson, C. ;
Carslaw, K. S. ;
Dalvi, M. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2013, 13 (06) :3027-3044
[5]   Bottom-up uncertainty estimates of global ammonia emissions from global agricultural production systems [J].
Beusen, A. H. W. ;
Bouwman, A. F. ;
Heuberger, P. S. C. ;
Van Drecht, G. ;
Van Der Hoek, K. W. .
ATMOSPHERIC ENVIRONMENT, 2008, 42 (24) :6067-6077
[6]   A global high-resolution emission inventory for ammonia [J].
Bouwman, AF ;
Lee, DS ;
Asman, WAH ;
Dentener, FJ ;
VanderHoek, KW ;
Olivier, JGJ .
GLOBAL BIOGEOCHEMICAL CYCLES, 1997, 11 (04) :561-587
[7]   How a century of ammonia synthesis changed the world [J].
Erisman, Jan Willem ;
Sutton, Mark A. ;
Galloway, James ;
Klimont, Zbigniew ;
Winiwarter, Wilfried .
NATURE GEOSCIENCE, 2008, 1 (10) :636-639
[8]   The need for ammonia abatement with respect to secondary PM reductions in Europe [J].
Erisman, JW ;
Schaap, M .
ENVIRONMENTAL POLLUTION, 2004, 129 (01) :159-163
[9]   ISORROPIA II:: a computationally efficient thermodynamic equilibrium model for K+-Ca2+-Mg2+-Nh4+-Na+-SO42--NO3--Cl--H2O aerosols [J].
Fountoukis, C. ;
Nenes, A. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2007, 7 (17) :4639-4659
[10]   Transformation of the nitrogen cycle: Recent trends, questions, and potential solutions [J].
Galloway, James N. ;
Townsend, Alan R. ;
Erisman, Jan Willem ;
Bekunda, Mateete ;
Cai, Zucong ;
Freney, John R. ;
Martinelli, Luiz A. ;
Seitzinger, Sybil P. ;
Sutton, Mark A. .
SCIENCE, 2008, 320 (5878) :889-892