Graphene Plasmonics: A Platform for Strong Light-Matter Interactions

被引:2325
作者
Koppens, Frank H. L. [1 ]
Chang, Darrick E. [2 ]
Javier Garcia de Abajo, F. [3 ,4 ]
机构
[1] ICFO Inst Ciencies Foton, Castelldefels 08860, Barcelona, Spain
[2] CALTECH, Pasadena, CA 91125 USA
[3] CSIC, Inst Opt, E-28006 Madrid, Spain
[4] Univ Southampton, Optoelect Res Ctr, Southampton SO17 1BJ, Hants, England
基金
英国工程与自然科学研究理事会;
关键词
graphene; plasmons; strong light-matter interaction; quantum optics; vacuum Rabi splitting; ENHANCED RAMAN-SCATTERING; SINGLE QUANTUM-DOT;
D O I
10.1021/nl201771h
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Graphene plasmons provide a suitable alternative to noble-metal plasmons because they exhibit much tighter confinement and relatively long propagation distances, with the advantage of being highly tunable via electrostatic gating. Here, we propose to use graphene plasmons as a platform for strongly enhanced light-matter interactions. Specifically, we predict unprecedented high decay rates of quantum emitters in the proximity of a carbon sheet, observable vacuum Rabi splittings, and extinction cross sections exceeding the geometrical area in graphene nanoribbons and nanodisks. Our theoretical results provide the basis for the emerging and potentially far-reaching field of graphene plasmonics, offering an ideal platform for cavity quantum electrodynamics, and supporting the possibility of single-molecule, single-plasmon devices.
引用
收藏
页码:3370 / 3377
页数:8
相关论文
共 55 条
[1]  
Atwater HA, 2010, NAT MATER, V9, P205, DOI [10.1038/nmat2629, 10.1038/NMAT2629]
[2]   Low Temperature Raman Study of the Electron Coherence Length near Graphene Edges [J].
Beams, Ryan ;
Cancado, Luiz Gustavo ;
Novotny, Lukas .
NANO LETTERS, 2011, 11 (03) :1177-1181
[3]   Electronic confinement and coherence in patterned epitaxial graphene [J].
Berger, Claire ;
Song, Zhimin ;
Li, Xuebin ;
Wu, Xiaosong ;
Brown, Nate ;
Naud, Cecile ;
Mayou, Didier ;
Li, Tianbo ;
Hass, Joanna ;
Marchenkov, Atexei N. ;
Conrad, Edward H. ;
First, Phillip N. ;
de Heer, Wait A. .
SCIENCE, 2006, 312 (5777) :1191-1196
[4]   Ultrahigh electron mobility in suspended graphene [J].
Bolotin, K. I. ;
Sikes, K. J. ;
Jiang, Z. ;
Klima, M. ;
Fudenberg, G. ;
Hone, J. ;
Kim, P. ;
Stormer, H. L. .
SOLID STATE COMMUNICATIONS, 2008, 146 (9-10) :351-355
[5]  
Bonaccorso F, 2010, NAT PHOTONICS, V4, P611, DOI [10.1038/nphoton.2010.186, 10.1038/NPHOTON.2010.186]
[6]   Observation of Plasmarons in Quasi-Freestanding Doped Graphene [J].
Bostwick, Aaron ;
Speck, Florian ;
Seyller, Thomas ;
Horn, Karsten ;
Polini, Marco ;
Asgari, Reza ;
MacDonald, Allan H. ;
Rotenberg, Eli .
SCIENCE, 2010, 328 (5981) :999-1002
[7]   The electronic properties of graphene [J].
Castro Neto, A. H. ;
Guinea, F. ;
Peres, N. M. R. ;
Novoselov, K. S. ;
Geim, A. K. .
REVIEWS OF MODERN PHYSICS, 2009, 81 (01) :109-162
[8]   Quantum optics with surface plasmons [J].
Chang, D. E. ;
Sorensen, A. S. ;
Hemmer, P. R. ;
Lukin, M. D. .
PHYSICAL REVIEW LETTERS, 2006, 97 (05)
[9]   Controlling inelastic light scattering quantum pathways in graphene [J].
Chen, Chi-Fan ;
Park, Cheol-Hwan ;
Boudouris, Bryan W. ;
Horng, Jason ;
Geng, Baisong ;
Girit, Caglar ;
Zettl, Alex ;
Crommie, Michael F. ;
Segalman, Rachel A. ;
Louie, Steven G. ;
Wang, Feng .
NATURE, 2011, 471 (7340) :617-620
[10]   Graphene nano-ribbon electronics [J].
Chen, Zhihong ;
Lin, Yu-Ming ;
Rooks, Michael J. ;
Avouris, Phaedon .
PHYSICA E-LOW-DIMENSIONAL SYSTEMS & NANOSTRUCTURES, 2007, 40 (02) :228-232