Hydrogen sulfide removal from natural gas using membrane technology: a review

被引：78

作者：

Ma, Yulei ^{[1
,2
,3
]}

Guo, Hongfang ^{[1
,2
,3
]}

Selyanchyn, Roman ^{[4
,5
]}

Wang, Bangda ^{[1
,2
,3
]}

Deng, Liyuan ^{[6
]}

Dai, Zhongde ^{[1
,2
,3
]}

Jiang, Xia ^{[1
,2
,3
]}

机构：

[1] Sichuan Univ, Coll Architecture & Environm, Chengdu 610065, Peoples R China

[2] Natl Engn Res Ctr Flue Gas Desulfurizat, Chengdu 610065, Peoples R China

[3] Carbon Neutral Technol Innovat Ctr Sichuan, Chengdu 610065, Peoples R China

[4] Kyushu Univ, Int Inst Carbon Neutral Energy Res WPI I2CNER, Nishi Ku, 744 Motooka, Fukuoka 8190395, Japan

[5] Kyushu Univ, Res Ctr Negat Emiss Technol, Nishi Ku, 744 Motooka, Fukuoka 8190395, Japan

[6] Norwegian Univ Sci & Technol, Dept Chem Engn, NO-7491 Trondheim, Norway

来源：

JOURNAL OF MATERIALS CHEMISTRY A | 2021年 / 9卷 / 36期

基金：

国家重点研发计划; 中国国家自然科学基金;

关键词：

HOLLOW-FIBER MEMBRANES; MIXED MATRIX MEMBRANE; METAL-ORGANIC FRAMEWORKS; CO-POLYIMIDE MEMBRANES; PHENOLIC IONIC LIQUIDS; HIGH-PRESSURE PURE; INTRINSIC MICROPOROSITY; CARBON-DIOXIDE; POLYMERIC MEMBRANES; TRANSPORT-PROPERTIES;

D O I：

10.1039/d1ta04693d

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Natural gas, having a significantly lower CO2 emission factor than oil and coal when combusted, is accepted as an important transition fuel towards carbon net-zero society. To meet the calorific value requirements (>= 34.0 MJ m(-3)) and reduce possible corrosion of transportation pipelines, acid gases such as CO2 and H2S must be removed from raw natural gas. Membrane separation is a promising alternative approach to remove acid gases from natural gas. This paper aims to review the development of various polymer-based membranes and membrane processes for H2S separation from natural gas. Progress in glassy polymer membranes, rubbery polymer membranes, hybrid membranes and membrane contactors for H2S removal from natural gas is summarized and analyzed. The H2S separation performance of various membranes is plotted in one diagram and a new H2S/CH4 upper bound is proposed. Challenges of membranes for H2S separation and prospects of future development are thoroughly discussed.

引用

页码：20211 / 20240

页数：30

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