Experiments and simulations on Al-Au mixtures and mixtures laws

被引:24
作者
Clerouin, Jean [1 ]
Recoules, Vanina [1 ]
Mazevet, Stephane [1 ]
Noiret, Pierre [1 ]
Renaudin, Patrick [1 ]
机构
[1] CEA, DAM, Dept Phys Theor & Appl, F-91680 Bruyeres Le Chatel, France
关键词
D O I
10.1103/PhysRevB.76.064204
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We measured the thermodynamical and transport properties of aluminum-gold mixtures in the warm dense matter regime and for various concentrations. We compare these measurements with quantum molecular dynamics (QMD) simulations. We find that the calculated pressures and resistivities of both the mixtures and pure phases are in good agreement with the measurements. This further allows us to test the mixing rules usually employed to predict the properties of the mixed phases from the pure ones. We show, in this regime, that the partial densities mixing rule predicts the pressure of the mixture rather accurately but fails in its prediction of the optical conductivity. To improve this latter prediction, we find that we must invoke an isothermal-isobaric mixture rule to compute the pure phase contributions at the correct densities.
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页数:8
相关论文
共 21 条
[1]   Viscosity and mutual diffusion in strongly asymmetric binary ionic mixtures [J].
Bastea, S .
PHYSICAL REVIEW E, 2005, 71 (05)
[2]  
Bushman A. V., 1992, EQUATION STATE METAL
[3]   GROUND-STATE OF THE ELECTRON-GAS BY A STOCHASTIC METHOD [J].
CEPERLEY, DM ;
ALDER, BJ .
PHYSICAL REVIEW LETTERS, 1980, 45 (07) :566-569
[4]   Electrical conductivity for warm, dense aluminum plasmas and liquids [J].
Desjarlais, MP ;
Kress, JD ;
Collins, LA .
PHYSICAL REVIEW E, 2002, 66 (02)
[5]   Electrical conductivity of warm expanded Al [J].
Faussurier, G ;
Blancard, C ;
Renaudin, P ;
Silvestrelli, PL .
PHYSICAL REVIEW B, 2006, 73 (07)
[6]  
GUILLOT T, 1999, SPACE SCI, V47
[7]  
GUILLOT T, 2003, INTERIOR JUPITER
[8]   EXPERIMENTS ON EXPANDED METALS IN THE METAL NONMETAL TRANSITION REGION [J].
HENSEL, F .
PHYSICA SCRIPTA, 1989, T25 :283-289
[9]  
HENSEL F, 1999, FLUID METALS
[10]   MISCIBILITY OF IONIZED IRON ATOMS IN HYDROGEN PLASMAS UNDER THE SOLAR INTERIOR CONDITIONS [J].
IYETOMI, H ;
ICHIMARU, S .
PHYSICAL REVIEW A, 1986, 34 (04) :3203-3209