Coherent control over Liouville-space pathways interference in transient four-wave mixing spectroscopy

被引：39

作者：

Pshenichnikov, MS

deBoeij, WP

Wiersma, DA

机构：

[1] Ultrafast Laser and Spectroscopy Laboratory, Department of Chemistry, Materials Science Centre, University of Groningen, Groningen, 9747 AG

来源：

PHYSICAL REVIEW LETTERS | 1996年 / 76卷 / 25期

关键词：

D O I：

10.1103/PhysRevLett.76.4701

中图分类号：

O4 [物理学];

学科分类号：

0702 ;

摘要：

A novel interference effect in transient four-wave mixing is demonstrated. The phenomenon is based on phase-controlled Liouville-space pathways interference and observed in the heterodyne-detected stimulated photon echo. Changing the phase difference between the first two excitation pulses from pi/2 to 0 leads from no signal to maximum echo signal. A Brownian oscillator dynamical model is successfully used to analyze the effect and simulate the experimental data. The relation between this time-domain interference effect and dephasing-induced resonance in four-wave mixing spectroscopy is elaborated.

引用

页码：4701 / 4704

页数：4

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